Tuning the Intrinsic Properties of Carbon Nitride for High Quantum Yield Photocatalytic Hydrogen Production.

作者: Mohammad Z. Rahman , Kenneth Davey , C. Buddie Mullins

DOI: 10.1002/ADVS.201800820

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摘要: The low quantum yield of photocatalytic hydrogen production in carbon nitride (CN) has been improved upon via the modulation of both the extrinsic and intrinsic properties of the material. Although the modification of extrinsic properties has been widely investigated in the past, recently there has been growing interest in the alteration of intrinsic properties. Refining the intrinsic properties of CN provides flexibility in controlling the charge transport and selectivity in photoredox reactions, and therefore makes available a pathway toward …

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