Plasma Nitrogen Oxides Synthesis in a Milli-Scale Gliding Arc Reactor: Investigating the Electrical and Process Parameters
作者： B. S. Patil , J. Rovira Palau , V. Hessel , Jürgen Lang , Q. Wang
DOI: 10.1007/S11090-015-9671-4
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摘要: Nitrogen fixed in the form of nitrogen oxides is essential to produce fertilizers and many other chemical products, which vital sustain life. The performance a milli-scale gliding arc reactor operated under atmospheric pressure has been studied for synthesis. In this work, electrical process parameters reactor, such as frequency, pulse width, amplitude feed ratio were investigated respectively. experiments performed at 1 L/min discharge regime. highest concentration NOx was found be ~1 % energy consumption 10 kWh/kg NOx. Increase width resulted an increased specific input concentration. (N2/O2) affected amount NO NO2 produced, gives possibility independently obtain desired NO/NO2 by tuning parameters.
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Krzysztof Krawczyk, Bogdan Ulejczyk, Decomposition of Chloromethanes in Gliding Discharges Plasma Chemistry and Plasma Processing. ,vol. 23, pp. 265- 281 ,(2003) , 10.1023/A:1022916018245
Z. Czekalska, Gases Conversion in Low Temperature Plasma Archivum Combustionis. pp. 337- 346 ,(2010)
Alexander Fridman, Plasma Chemistry Cambridge University Press. ,(2008) , 10.1017/CBO9780511546075
Muhammad Arif Malik, Chunqi Jiang, Richard Heller, Jamie Lane, David Hughes, Karl H. Schoenbach, Ozone-free nitric oxide production using an atmospheric pressure surface discharge – A way to minimize nitrogen dioxide co-production Chemical Engineering Journal. ,vol. 283, pp. 631- 638 ,(2016) , 10.1016/J.CEJ.2015.07.092
Olivier Aubry, Ahmed Khacef, Jean Marie Cormier, Degradation of Organics Compounds and Production of Activated Species in Dielectric Barrier Discharges and Glidarc Reactors NATO-Advanced Study Institute on Plasma Assisted Decontamination of biological and Chemical Agents. pp. 125- 134 ,(2008) , 10.1007/>978-1-4020-8439-3_10
V. Dalaine, J. M. Cormier, P. Lefaucheux, A gliding discharge applied to H2S destruction Journal of Applied Physics. ,vol. 83, pp. 2435- 2441 ,(1998) , 10.1063/1.367003
B.S. Patil, Q. Wang, V. Hessel, J. Lang, Plasma N2-fixation : 1900-2014 Catalysis Today. ,vol. 256, pp. 49- 66 ,(2015) , 10.1016/J.CATTOD.2015.05.005
Max Appl, Ammonia, 2. Production Processes Ullmann's Encyclopedia of Industrial Chemistry. ,(2011) , 10.1002/14356007.O02_O11
A. Czernichowski, Gliding arc: Applications to engineering and environment control Pure and Applied Chemistry. ,vol. 66, pp. 1301- 1310 ,(1994) , 10.1351/PAC199466061301
A INDARTO, J CHOI, H LEE, H SONG, Effect of additive gases on methane conversion using gliding arc discharge Energy. ,vol. 31, pp. 2986- 2995 ,(2006) , 10.1016/J.ENERGY.2005.10.034