Study of initial stages of thin film growth by means of atomistic computer simulation and image analysis: Comparison with experimental data

作者: Rudolf Hrach , Dušan Novotný , Stanislav Novák

DOI: 10.1016/J.VACUUM.2018.01.006

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摘要: Abstract The initial stages of metal film growth were studied by computer experiment. structures generated an atomistic model combining the molecular dynamics and Monte Carlo approaches analysis obtained was performed image processing algorithms. Film morphology tested several methods it found that especially Voronoi tessellation Quadrat Counts are best suited for a description spatial distribution objects. same morphological applied to experimental data – micrographs discontinuous films Ag, Au In grown on dielectric or graphite substrates. It small evaporation rates is in good agreement with experiments. However, when increasing effect secondary nucleation starts be pronounced discrepancy between modelled experimentally derived results occurs. This demonstrated indium intensive nucleation.

参考文章(36)
Feng Shi, Yunsic Shim, Jacques G. Amar, Parallel kinetic Monte Carlo simulations of two-dimensional island coarsening Physical Review E. ,vol. 76, pp. 031607- ,(2007) , 10.1103/PHYSREVE.76.031607
V. Senthil Kumar, V. Kumaran, Voronoi neighbor statistics of homogeneously sheared inelastic hard disks and hard spheres. Physical Review E. ,vol. 73, pp. 051305- ,(2006) , 10.1103/PHYSREVE.73.051305
A. Sedehi, Z.H. Meiksin, J.R. Blachere, Real-time simulation of nucleation and growth of vacuum-evaporated thin metallic films Thin Solid Films. ,vol. 98, pp. 49- 58 ,(1982) , 10.1016/0040-6090(82)90626-5
RY Yang, RP Zou, AB Yu, None, Voronoi tessellation of the packing of fine uniform spheres. Physical Review E. ,vol. 65, pp. 041302- ,(2002) , 10.1103/PHYSREVE.65.041302
E Dobierzewska-Mozrzymas, P Biegański, G Szymczak, Microstructures of island metal films—the computer simulations and statistical description Vacuum. ,vol. 63, pp. 59- 65 ,(2001) , 10.1016/S0042-207X(01)00171-3
Eloi Pineda, Victor Garrido, Daniel Crespo, Domain-size distribution in a Poisson-Voronoi nucleation and growth transformation. Physical Review E. ,vol. 75, pp. 040107- ,(2007) , 10.1103/PHYSREVE.75.040107
Martin Mašín, Miroslav Kotrla, Influence of control and material parameters on island density in early stage of pulsed laser deposition Thin Solid Films. ,vol. 520, pp. 4965- 4970 ,(2012) , 10.1016/J.TSF.2012.03.021
P. Biegański, E. Dobierzewska-Mozrzymas, E. Pieciul, G. Szymczak, Influence of microstructure on the conduction mechanisms in discontinuous metal films on dielectric substrates Vacuum. ,vol. 74, pp. 211- 216 ,(2004) , 10.1016/J.VACUUM.2003.12.124
B. Pauwels, G. Van Tendeloo, W. Bouwen, L. Theil Kuhn, P. Lievens, H. Lei, M. Hou, Low-energy-deposited Au clusters investigated by high-resolution electron microscopy and molecular dynamics simulations Physical Review B. ,vol. 62, pp. 10383- 10393 ,(2000) , 10.1103/PHYSREVB.62.10383
Witold Brostow, Mieczyslaw Chybicki, Robert Laskowski, Jaroslaw Rybicki, Voronoi polyhedra and Delaunay simplexes in the structural analysis of molecular-dynamics-simulated materials Physical Review B. ,vol. 57, pp. 13448- 13458 ,(1998) , 10.1103/PHYSREVB.57.13448