Formal total synthesis of (+)-trehazolin. Application of an asymmetric aldol-olefin metathesis approach to the synthesis of functionalized cyclopentenes.

作者： Michael T. Crimmins , Elie A. Tabet

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摘要: An asymmetric synthesis of the aminocyclopentitol pseudosugar trehazolin has been completed. The hinges on an aldol-ring closing metathesis strategy to construct five-membered ring with control both relative and absolute stereochemistry.

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Formal total synthesis of (+)-trehazolin. Application of an asymmetric aldol-olefin metathesis approach to the synthesis of functionalized cyclopentenes.

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Formal total synthesis of (+)-trehazolin. Application of an asymmetric aldol-olefin metathesis approach to the synthesis of functionalized cyclopentenes.

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