Generalized Förster-Dexter theory of photoinduced intramolecular energy transfer

作者: S. H. Lin , W. Z. Xiao , W. Dietz

DOI: 10.1103/PHYSREVE.47.3698

关键词:

摘要: In this paper, we generalize the F\"orster-Dexter theory to treat photoinduced electronic energy transfer for a system in dense media and an isolated (i.e., collision-free condition). Instead of expressing rate terms spectral overlap, obtain expression energy-transfer constant by evaluating Fourier integral using saddle-point method. way, energy-gap dependence effect temperature isotope on can be easily studied. The bridge groups connecting between donor acceptor is also

参考文章(20)
R.M. Macfarlane, R.M. Shelby, Measurement of optical dephasing of Eu3+ and Pr3+ doped silicate glasses by spectral holeburning Optics Communications. ,vol. 45, pp. 46- 51 ,(1983) , 10.1016/0030-4018(83)90407-8
R.M. MacFarlane, R.M. Shelby, Homogeneous line broadening of optical transitions of ions and molecules in glasses Journal of Luminescence. ,vol. 36, pp. 179- 207 ,(1987) , 10.1016/0022-2313(87)90194-3
Christopher S. Foote, Robert W. Denny, CHEMISTRY OF SINGLET OXYGEN. VII QUENCHING BY B – CAROTENE Journal of the American Chemical Society. ,vol. 90, pp. 6233- 6235 ,(1968) , 10.1021/JA01024A061
Richard J. Cogdell, Harry A. Frank, How carotenoids function in photosynthetic bacteria. Biochimica et Biophysica Acta. ,vol. 895, pp. 63- 79 ,(1987) , 10.1016/S0304-4173(87)80008-3
Thomas A. Moore, Devens Gust, Susan Hatlevig, Ana L. Moore, Lewis R. Makings, Peter J. Pesski, F.C. De Schryver, M. van Der Auweraer, Doris Lexa, René V. Bensasson, Michel Rougée, Photoinitiated Electron Transfer in Carotenoporphyrin-Quinone Triads: Enhanced Quantum Yields via Control of Reaction Exergonicity Israel Journal of Chemistry. ,vol. 28, pp. 87- 95 ,(1988) , 10.1002/IJCH.198800017
Richard Snyder, Eric Arvidson, Caroline Foote, Lynne Harrigan, Ronald L. Christensen, Electronic energy levels in long polyenes: S2 .fwdarw. S0 emission in all-trans-1,3,5,7,9,11,13-tetradecaheptaene Journal of the American Chemical Society. ,vol. 107, pp. 4117- 4122 ,(1985) , 10.1021/JA00300A004
GODFREY S. BEDDARD, R. STEPHEN DAVIDSON, KENNETH R. TRETHEWEY, Quenching of chlorophyll fluorescence by β-carotene Nature. ,vol. 267, pp. 373- 374 ,(1977) , 10.1038/267373A0
Barbara Demmig-Adams, Carotenoids and photoprotection in plants : a role for the xanthophyll zeaxanthin Biochimica et Biophysica Acta. ,vol. 1020, pp. 1- 24 ,(1990) , 10.1016/0005-2728(90)90088-L
Devens Gust, Thomas A. Moore, Ana L. Moore, Chelladurai Devadoss, Paul A. Liddell, Roel Hermant, Ronald A. Nieman, Lori J. Demanche, Janice M. DeGraziano, Isabelle Gouni, Triplet and singlet energy transfer in carotene-porphyrin dyads: role of the linkage bonds. Journal of the American Chemical Society. ,vol. 114, pp. 3590- 3603 ,(1992) , 10.1021/JA00036A002