Nanoscale Transient Magnetization Gratings Created and Probed by Femtosecond Extreme Ultraviolet Pulses.

作者: Flavio Capotondi , Stefano Bonetti , Stefano Bonetti , Emanuele Pedersoli , Matteo Pancaldi

DOI: 10.1021/ACS.NANOLETT.0C05083

关键词:

摘要: We utilize coherent femtosecond extreme ultraviolet (EUV) pulses from a free electron laser (FEL) to generate transient periodic magnetization patterns with periods as short 44 nm. Combining spatially excitation resonant probing at the M-edge of cobalt allows us create and probe gratings electronic magnetic excitations in CoGd alloy. In demagnetized sample, we observe an rise time close FEL pulse duration ∼0.5 ps decay indicative electron-phonon relaxation. When sample is magnetized saturation external field, grating, which appears on subpicosecond scale maxima EUV intensity then decays tens picoseconds via thermal diffusion. The described approach opens multiple avenues for studying dynamics ultrafast phenomena nanometer length scales.

参考文章(32)
Tian-Min Liu, Tianhan Wang, Alexander H. Reid, Matteo Savoini, Xiaofei Wu, Benny Koene, Patrick Granitzka, Catherine E. Graves, Daniel J. Higley, Zhao Chen, Gary Razinskas, Markus Hantschmann, Andreas Scherz, Joachim Stöhr, Arata Tsukamoto, Bert Hecht, Alexey V. Kimel, Andrei Kirilyuk, Theo Rasing, Hermann A. Dürr, Nanoscale Confinement of All-Optical Magnetic Switching in TbFeCo - Competition with Nanoscale Heterogeneity Nano Letters. ,vol. 15, pp. 6862- 6868 ,(2015) , 10.1021/ACS.NANOLETT.5B02743
C. von Korff Schmising, B. Pfau, M. Schneider, C. M. Günther, M. Giovannella, J. Perron, B. Vodungbo, L. Müller, F. Capotondi, E. Pedersoli, N. Mahne, J. Lüning, S. Eisebitt, Imaging Ultrafast Demagnetization Dynamics after a Spatially Localized Optical Excitation Physical Review Letters. ,vol. 111, pp. 217203- ,(2014) , 10.1103/PHYSREVLETT.112.217203
M. Battiato, K. Carva, P. M. Oppeneer, Superdiffusive Spin Transport as a Mechanism of Ultrafast Demagnetization Physical Review Letters. ,vol. 105, pp. 027203- 027203 ,(2010) , 10.1103/PHYSREVLETT.105.027203
E. Allaria, D. Castronovo, P. Cinquegrana, P. Craievich, M. Dal Forno, M. B. Danailov, G. D'Auria, A. Demidovich, G. De Ninno, S. Di Mitri, B. Diviacco, W. M. Fawley, M. Ferianis, E. Ferrari, L. Froehlich, G. Gaio, D. Gauthier, L. Giannessi, R. Ivanov, B. Mahieu, N. Mahne, I. Nikolov, F. Parmigiani, G. Penco, L. Raimondi, C. Scafuri, C. Serpico, P. Sigalotti, S. Spampinati, C. Spezzani, M. Svandrlik, C. Svetina, M. Trovo, M. Veronese, D. Zangrando, M. Zangrando, Two-stage seeded soft-X-ray free-electron laser Nature Photonics. ,vol. 7, pp. 913- 918 ,(2013) , 10.1038/NPHOTON.2013.277
Todd S. Rose, William L. Wilson, G. Wäckerle, M. D. Fayer, Gas phase dynamics and spectroscopy probed with picosecond transient grating experiments The Journal of Chemical Physics. ,vol. 86, pp. 5370- 5391 ,(1987) , 10.1063/1.452773
Andrei Kirilyuk, Alexey V Kimel, Theo Rasing, Laser-induced magnetization dynamics and reversal in ferrimagnetic alloys. Reports on Progress in Physics. ,vol. 76, pp. 026501- ,(2013) , 10.1088/0034-4885/76/2/026501
V. López-Flores, N. Bergeard, V. Halté, C. Stamm, N. Pontius, M. Hehn, E. Otero, E. Beaurepaire, C. Boeglin, Role of critical spin fluctuations in ultrafast demagnetization of transition-metal rare-earth alloys Physical Review B. ,vol. 87, pp. 214412- ,(2013) , 10.1103/PHYSREVB.87.214412
K Shirakawa, K Fukamichi, K Aoki, T Masumoto, T Kaneko, The Curie temperature of amorphous and crystalline Gd−Co alloys and its pressure effect Journal of Physics F: Metal Physics. ,vol. 15, pp. 961- 968 ,(1985) , 10.1088/0305-4608/15/4/020
Nuh Gedik, Anthony T. Bollinger, Fahad Mahmood, Darius H. Torchinsky, Ivan Božović, Fluctuating charge-density waves in a cuprate superconductor Nature Materials. ,vol. 12, pp. 387- 391 ,(2013) , 10.1038/NMAT3571
C. Gutt, S. Streit-Nierobisch, L.-M. Stadler, B. Pfau, C. M. Günther, R. Könnecke, R. Frömter, A. Kobs, D. Stickler, H. P. Oepen, R. R. Fäustlin, R. Treusch, J. Feldhaus, E. Weckert, I. A. Vartanyants, M. Grunze, A. Rosenhahn, T. Wilhein, S. Eisebitt, G. Grübel, Single-pulse resonant magnetic scattering using a soft x-ray free-electron laser Physical Review B. ,vol. 81, pp. 100401- ,(2010) , 10.1103/PHYSREVB.81.100401