Contributions of deposited particles to pine needle polycyclic aromatic hydrocarbons

作者: Ping Yang , Jingwen Chen , Zhen Wang , Xianliang Qiao , Xiyun Cai

DOI: 10.1039/B708508G

关键词:

摘要: The contributions of deposited particles (P) to polycyclic aromatic hydrocarbon (PAH) levels in pine (Cedrus deodar) needles sampled from the Dalian region were evaluated by washing off needle surfaces. P values ranged 4.4 ± 2.2% for fluorene 69.9 4.0% indeno(1,2,3-cd)pyrene, and positively correlated with logarithm octanol–air partition coefficients (log KOA) each PAH significantly. total 14 PAHs under study (∑PAHs), that 490 3241 ng g−1 dw (dry weight) median value 1521 dw, high traffic areas, low residential or park implying significant both gas particle phases emitted vehicles. However, profiles not significantly altered washing, due fractions (2–5%) 5- 6-ring ∑PAHs. wind speed frequently alternating directions spring could quicken depuration processes PAHs. Thus, local meteorological conditions source variations should be taken into account when using implicate seasonal atmospheric semi-volatile organic compounds.

参考文章(30)
Tom Harner, Terry F. Bidleman, Octanol−Air Partition Coefficient for Describing Particle/Gas Partitioning of Aromatic Compounds in Urban Air Environmental Science & Technology. ,vol. 32, pp. 1494- 1502 ,(1998) , 10.1021/ES970890R
Håkan Wingfors, Åke Sjödin, Peter Haglund, Eva Brorström-Lundén, Characterisation and determination of profiles of polycyclic aromatic hydrocarbons in a traffic tunnel in Gothenburg, Sweden Atmospheric Environment. ,vol. 35, pp. 6361- 6369 ,(2001) , 10.1016/S1352-2310(01)00389-2
Kilian E.C. Smith, Kevin C. Jones, Particles and vegetation: implications for the transfer of particle-bound organic contaminants to vegetation Science of The Total Environment. ,vol. 246, pp. 207- 236 ,(2000) , 10.1016/S0048-9697(99)00459-3
Michael S. McLachlan, Framework for the Interpretation of Measurements of SOCs in Plants Environmental Science & Technology. ,vol. 33, pp. 1799- 1804 ,(1999) , 10.1021/ES980831T
Michael S. McLachlan, Kerstin. Welsch-Pausch, Johannes. Tolls, Field Validation of a Model of the Uptake of Gaseous SOC in Lolium multiflorum (Welsh Ray Grass). Environmental Science & Technology. ,vol. 29, pp. 1998- 2004 ,(1995) , 10.1021/ES00008A018
Ioannis E. Sitaras, Evangelos B. Bakeas, Panayotis A. Siskos, Gas/particle partitioning of seven volatile polycyclic aromatic hydrocarbons in a heavy traffic urban area Science of The Total Environment. ,vol. 327, pp. 249- 264 ,(2004) , 10.1016/J.SCITOTENV.2003.08.022
Kilian E. C. Smith, Gareth O. Thomas, Kevin C. Jones, Seasonal and Species Differences in the Air−Pasture Transfer of PAHs Environmental Science & Technology. ,vol. 35, pp. 2156- 2165 ,(2001) , 10.1021/ES000200A
Staci L. Simonich, Ronald A. Hites, Organic pollutant accumulation in vegetation. Environmental Science & Technology. ,vol. 29, pp. 2905- 2914 ,(1995) , 10.1021/ES00012A004
Anne Motelay-Massei, Tom Harner, Mahiba Shoeib, Miriam Diamond, Gary Stern, Bruno Rosenberg, Using Passive Air Samplers To Assess Urban−Rural Trends for Persistent Organic Pollutants and Polycyclic Aromatic Hydrocarbons. 2. Seasonal Trends for PAHs, PCBs, and Organochlorine Pesticides Environmental Science & Technology. ,vol. 39, pp. 5763- 5773 ,(2005) , 10.1021/ES0504183