A density matrix approach to photoinduced electron injection

作者: Ivan Kondov , Michael Schreiber , Michael Schreiber , Ulrich Kleinekathöfer

DOI: 10.1016/S0022-2313(01)00341-6

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摘要: Abstract Electron injection from an adsorbed molecule to the substrate (heterogeneous electron transfer) is studied. One reaction coordinate used model this process. The surface phonons and/or electron–hole pairs together with internal degrees of freedom as well a liquid possibly surrounding provide dissipative environment, which may lead dephasing, relaxation, and sometimes excitation relevant system. In process studied, excited by light pulse. This followed transfer donor state quasi-continuum substrate. It assumed that semiconductor. effects dissipation on are investigated.

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