Spatio-temporal variations and factors of a provincial PM 2.5 pollution in eastern China during 2013–2017 by geostatistics

作者: Xue Sun , Xiao-San Luo , Jiangbing Xu , Zhen Zhao , Yan Chen

DOI: 10.1038/S41598-019-40426-8

关键词:

摘要: Fine particulate matter (PM2.5) is a typical air pollutant and has adverse health effects across the world, especially in rapidly developing China due to significant pollution. The PM2.5 pollution varies with time space, dominated by locations owing differences geographical conditions including topography meteorology, land use characteristics of urbanization industrialization, all which control formation influencing various sources transport PM2.5. To characterize these parameters mechanisms, 5-year patterns Jiangsu province eastern high-resolution was investigated. Kriging interpolation method geostatistical analysis (GIS) HYbrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model were conducted study spatial temporal distribution at 110 sites from national quality monitoring network covering 13 cities. studied region obvious, although annual average concentration decreased previous 72 recent 50 μg m−3. Evident variations showed high level winter low summer. Spatially, higher northern (inland, heavy industry) than that (costal, plain) regions. Industrial contributed highest Backward trajectory clustering potential source contribution factor (PSCF) indicated monsoon climate played an important role aerosol transport. In summer, mass mainly affected updraft near region, accounted for about 60% total number trajectories, while winter, long-distance northwest had impact on

参考文章(48)
Magdalena Reizer, Katarzyna Juda-Rezler, Explaining the high PM10 concentrations observed in Polish urban areas. Air Quality, Atmosphere & Health. ,vol. 9, pp. 517- 531 ,(2016) , 10.1007/S11869-015-0358-Z
Takashi Yorifuji, Sanghyuk Bae, Saori Kashima, Toshihide Tsuda, Hiroyuki Doi, Yasushi Honda, Ho Kim, Yun-Chul Hong, None, Health Impact Assessment of PM10 and PM2.5 in 27 Southeast and East Asian Cities. Journal of Occupational and Environmental Medicine. ,vol. 57, pp. 751- 756 ,(2015) , 10.1097/JOM.0000000000000485
Ukkyo Jeong, Jhoon Kim, Hanlim Lee, Jinsang Jung, Young J. Kim, Chul H. Song, Ja-Ho Koo, Estimation of the contributions of long range transported aerosol in East Asia to carbonaceous aerosol and PM concentrations in Seoul, Korea using highly time resolved measurements: a PSCF model approach Journal of Environmental Monitoring. ,vol. 13, pp. 1905- 1918 ,(2011) , 10.1039/C0EM00659A
Hong He, Yi Li, Xiuli Zhang, Yunbo Yu, Changbin Zhang, None, Precipitable silver compound catalysts for the selective catalytic reduction of NOx by ethanol Applied Catalysis A-general. ,vol. 375, pp. 258- 264 ,(2010) , 10.1016/J.APCATA.2010.01.002
Hong Xu, Xiao-Hui Bi, Wei-Wei Zheng, Jian-Hui Wu, Yin-Chang Feng, Particulate matter mass and chemical component concentrations over four Chinese cities along the western Pacific coast. Environmental Science and Pollution Research. ,vol. 22, pp. 1940- 1953 ,(2015) , 10.1007/S11356-014-3630-0
WY Xu, CS Zhao, L Ran, ZZ Deng, N Ma, PF Liu, WL Lin, P Yan, XB Xu, None, A new approach to estimate pollutant emissions based on trajectory modeling and its application in the North China Plain Atmospheric Environment. ,vol. 71, pp. 75- 83 ,(2013) , 10.1016/J.ATMOSENV.2013.01.047
Zhaoxi Wang, David C. Christiani, Petros Koutrakis, Yang Liu, Kebin He, Shenshen Li, A statistical model to evaluate the effectiveness of PM2.5 emissions control during the Beijing 2008 Olympic Games Environment International. ,vol. 44, pp. 100- 105 ,(2012) , 10.1016/J.ENVINT.2012.02.003
K. Křůmal, P. Mikuška, M. Vojtěšek, Z. Večeřa, Seasonal variations of monosaccharide anhydrides in PM1 and PM2.5 aerosol in urban areas Atmospheric Environment. ,vol. 44, pp. 5148- 5155 ,(2010) , 10.1016/J.ATMOSENV.2010.08.057
Kota Katanoda, Tomotaka Sobue, Hiroshi Satoh, Kazuo Tajima, Takaichiro Suzuki, Haruo Nakatsuka, Toshiro Takezaki, Tomio Nakayama, Hiroshi Nitta, Kiyoshi Tanabe, Suketami Tominaga, An Association Between Long-Term Exposure to Ambient Air Pollution and Mortality From Lung Cancer and Respiratory Diseases in Japan Journal of Epidemiology. ,vol. 21, pp. 132- 143 ,(2011) , 10.2188/JEA.JE20100098
L. T. Wang, Z. Wei, J. Yang, Y. Zhang, F. F. Zhang, J. Su, C. C. Meng, Q. Zhang, The 2013 severe haze over southern Hebei, China: model evaluation, source apportionment, and policy implications Atmospheric Chemistry and Physics. ,vol. 14, pp. 3151- 3173 ,(2014) , 10.5194/ACP-14-3151-2014