Atmospheric fate and transport of dioxins: local impacts.

作者: Kristen Lohman , Christian Seigneur

DOI: 10.1016/S0045-6535(00)00559-2

关键词:

摘要: We conducted model simulations of the atmospheric fate and transport PCDD/F to assess fraction emitted that would deposit within 100 km from source. considered eight major categories emission sources six different locations, cover a wide range source characteristics, congener profiles particle size distributions, meteorological conditions terrain configurations. These results suggest for have tall stacks and/or high plume rise (e.g., copper smelters, cement kilns, sinter plants), only small emissions is deposited locally (typically, less than 10% km). Other such as municipal solid waste incinerators, medical incinerators diesel trucks lead greater being locally; nevertheless, majority their tends be transported beyond km. Although local impacts may need addressed these latter categories, it appears long-range potential all categories. Sensitivity studies were investigate effect various key inputs on simulation results. an advanced dispersion should used cases where present some concerns because are very sensitive treatment dispersion. Also, essential obtain accurate characterizations distribution particulate dry deposition flux distribution.

参考文章(25)
Mark Z. Jacobson, Fundamentals of atmospheric modeling ,(1998)
P. K. Hopke, C. Seigneur, D. Grosjean, P. Pai, Modeling atmospheric particulate matter Environmental Science & Technology. ,vol. 33, ,(1999)
Tom Harner, Terry F. Bidleman, Octanol−Air Partition Coefficient for Describing Particle/Gas Partitioning of Aromatic Compounds in Urban Air Environmental Science & Technology. ,vol. 32, pp. 1494- 1502 ,(1998) , 10.1021/ES970890R
Paul M. Lemieux, Christopher C. Lutes, Judith A. Abbott, Kenneth M. Aldous, Emissions of polychlorinated dibenzo-p-dioxins and polychlorinated dibenzofurans from the open burning of household waste in barrels Environmental Science & Technology. ,vol. 34, pp. 377- 384 ,(2000) , 10.1021/ES990465T
J.P. Basham, I. Whitwell, Dispersion modelling of dioxin releases from the waste incinerator at Avonmouth, Bristol, UK Atmospheric Environment. ,vol. 33, pp. 3405- 3416 ,(1999) , 10.1016/S1352-2310(98)00344-6
R. I. Sykes, S. F. Parker, D. S. Henn, W. S. Lewellen, Numerical Simulation of ANATEX Tracer Data Using a Turbulence Closure Model for Long-Range Dispersion Journal of Applied Meteorology. ,vol. 32, pp. 929- 947 ,(1993) , 10.1175/1520-0450(1993)032<0929:NSOATD>2.0.CO;2
Prakash Karamchandani, Lynne Santos, Ian Sykes, Yang Zhang, Cathryn Tonne, Christian Seigneur, Development and Evaluation of a State-of-the-Science Reactive Plume Model Environmental Science & Technology. ,vol. 34, pp. 870- 880 ,(2000) , 10.1021/ES990611V
John I. Baker, Ronald A. Hites, Polychlorinated dibenzo-p-dioxins and dibenzofurans in the remote North Atlantic marine atmosphere Environmental Science & Technology. ,vol. 33, pp. 14- 20 ,(1999) , 10.1021/ES980369C
Yoichi Kurokawa, Matsueda Takahiko, Nakamura Matayoshi, Takada Satoshi, Fukamachi Kazumi, Distribution of polychlorinated dibenzo-p-dioxins and dibenzofurans in various sizes of airborne particles Chemosphere. ,vol. 37, pp. 2161- 2171 ,(1998) , 10.1016/S0045-6535(98)00278-1