Experimental investigation of liquid water formation and transport in a transparent single-serpentine PEM fuel cell

作者: Dusan Spernjak , Ajay K. Prasad , Suresh G. Advani

DOI: 10.1016/J.JPOWSOUR.2007.04.020

关键词:

摘要: Liquid water formation and transport were investigated by direct experimental visualization in an operational transparent single-serpentine PEM fuel cell. We examined the effectiveness of various gas diffusion layer (GDL) materials removing away from cathode through flow field over a range operating conditions. Complete polarization curves as well time evolution studies after step changes current draw obtained with simultaneous liquid within The level flooding, under same conditions cell current, was recognized criterion for removal capacity GDL materials. When compared at density (i.e. production rate), higher amount channel indicated that had been efficiently removed catalyst layer. Visualization anode used to investigate influence microporous (MPL) on transport. No observed unless GDLs MPL. MPL side creates pressure barrier produced layer. Water is pushed across membrane side, resulting flooding close H2 exit.

参考文章(20)
Hubert Gasteiger, Wolf Vielstich, Arnold Lamm, Handbook of fuel cells : fundamentals technology and applications Wiley. ,(2003)
Alex Hakenjos, Harald Muenter, Ursula Wittstadt, Christopher Hebling, A PEM fuel cell for combined measurement of current and temperature distribution, and flow field flooding Journal of Power Sources. ,vol. 131, pp. 213- 216 ,(2004) , 10.1016/J.JPOWSOUR.2003.11.081
P. Concus, R. Finn, ON THE BEHAVIOR OF A CAPILLARY SURFACE IN A WEDGE Proceedings of the National Academy of Sciences of the United States of America. ,vol. 63, pp. 292- 299 ,(1969) , 10.1073/PNAS.63.2.292
James Larminie, Andrew Dicks, Maurice S McDonald, Fuel cell systems explained ,(2000)
Zhigang Qi, Arthur Kaufman, Enhancement of PEM fuel cell performance by steaming or boiling the electrode Journal of Power Sources. ,vol. 109, pp. 227- 229 ,(2002) , 10.1016/S0378-7753(02)00060-5
X. G. Yang, F. Y. Zhang, A. L. Lubawy, C. Y. Wang, Visualization of Liquid Water Transport in a PEFC Electrochemical and Solid State Letters. ,vol. 7, ,(2004) , 10.1149/1.1803051
Shohji Tsushima, Kazuhiro Teranishi, Shuichiro Hirai, Magnetic Resonance Imaging of the Water Distribution within a Polymer Electrolyte Membrane in Fuel Cells Electrochemical and Solid State Letters. ,vol. 7, ,(2004) , 10.1149/1.1774971
F BARBIR, H GORGUN, X WANG, Relationship between pressure drop and cell resistance as a diagnostic tool for PEM fuel cells Journal of Power Sources. ,vol. 141, pp. 96- 101 ,(2005) , 10.1016/J.JPOWSOUR.2004.08.055
Zhigang Qi, Arthur Kaufman, Improvement of water management by a microporous sublayer for PEM fuel cells Journal of Power Sources. ,vol. 109, pp. 38- 46 ,(2002) , 10.1016/S0378-7753(02)00058-7
J. Martin, P. Oshkai, N. Djilali, Flow Structures in a U-Shaped Fuel Cell Flow Channel: Quantitative Visualization Using Particle Image Velocimetry Journal of Fuel Cell Science and Technology. ,vol. 2, pp. 70- 80 ,(2005) , 10.1115/1.1843121