Electric-Field-Mediated Electron Tunneling of Supramolecular Naphthalimide Nanostructures for Biomimetic H2 Production.
作者： Junhui Wang , Kaifeng Wu , Huaping Jia , Xuming Zhang , Xinhua Cao
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摘要: The design and synthesis of two semiconducting bis (4‐ethynyl‐bridging 1, 8‐naphthalimide) bolaamphiphiles (BENI‐COO− and BENI‐NH3+) to fabricate supramolecular metal–insulator–semiconductor (MIS) nanostructures for biomimetic hydrogen evolution under visible light irradiation is presented. A H2 evolution rate of ca. 3.12 mmol g− 1⋅ h− 1 and an apparent quantum efficiency (AQE) of ca. 1.63% at 400 nm were achieved over the BENI‐COO−‐NH3+‐Ni MIS photosystem prepared by electrostatic self‐assembly of BENI …
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