Tuning the wavelength of amplified spontaneous emission coupled to localized surface plasmon

作者: S. Murai , Y. Tokuda , K. Fujita , K. Tanaka

DOI: 10.1063/1.4736408

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摘要: Amplified spontaneous emissions (ASEs) with a tuned wavelength have been observed in thin film composite made by spin-coating dye-doped polymer layer (thickness ∼80 nm) on Ag nanoparticles deposited SiO2 substrate. The samples having varied of the localized surface plasmon resonance (LSPR) are excited second harmonic pulses from Nd3+ doped yttrium aluminum garnet laser. When pump energy exceeds threshold, spectrally narrow peak appears broad emission dye molecules nonlinear increase intensity, indicating an onset ASE. It is found that ASE shifts change LSPR.

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