Field-Driven Quantum Criticality in the Spinel Magnet ZnCr 2 Se 4

作者: CC Gu , ZY Zhao , XL Chen , M Lee , ES Choi

DOI: 10.1103/PHYSREVLETT.120.147204

关键词:

摘要: We report detailed dc and ac magnetic susceptibilities, specific heat, thermal conductivity measurements on the frustrated magnet ${\mathrm{ZnCr}}_{2}{\mathrm{Se}}_{4}$. At low temperatures, with an increasing field, this spinel material goes through a series of spin state transitions from helix to spiral then fully polarized state. Our results indicate direct quantum phase transition As system approaches criticality, we find strong fluctuations spins behaviors such as unconventional ${T}^{2}$-dependent heat temperature-independent mean free path for transport. complete full diagram ${\mathrm{ZnCr}}_{2}{\mathrm{Se}}_{4}$ under external field propose possibility criticality extended densities critical modes account unusual low-energy excitations in vicinity criticality. reveal that is rare example 3D exhibiting field-driven properties.

参考文章(35)
Tian Liang, S. M. Koohpayeh, J. W. Krizan, T. M. McQueen, R. J. Cava, N. P. Ong, Heat capacity peak at the quantum critical point of the transverse Ising magnet CoNb2O6 Nature Communications. ,vol. 6, pp. 7611- 7611 ,(2015) , 10.1038/NCOMMS8611
Jun Akimitsu, Kiiti Siratori, Gen Shirane, Masashi Iizumi, Tsuneo Watanabe, Neutron Scattering Study of ZnCr2Se4 with Screw Spin Structure Journal of the Physical Society of Japan. ,vol. 44, pp. 172- 180 ,(1978) , 10.1143/JPSJ.44.172
Gang Chen, Andreas P. Schnyder, Leon Balents, Excitation spectrum and magnetic field effects in a quantum critical spin-orbital system: The case of FeSc 2 S 4 Physical Review B. ,vol. 80, pp. 224409- ,(2009) , 10.1103/PHYSREVB.80.224409
O. Tchernyshyov, S. M. Koohpayeh, J. Krizan, T. M. McQueen, R. Valdés Aguilar, R. J. Cava, N. P. Armitage, C. M. Morris, A. Ghosh, A hierarchy of bound states in the 1D ferromagnetic Ising chain CoNb$_2$O$_6$ investigated by high resolution time-domain terahertz spectroscopy arXiv: Strongly Correlated Electrons. ,(2013) , 10.1103/PHYSREVLETT.112.137403
T. Rudolf, Ch. Kant, F. Mayr, J. Hemberger, V. Tsurkan, A. Loidl, Spin-phonon coupling in Zn Cr 2 Se 4 Physical Review B. ,vol. 75, pp. 052410- ,(2007) , 10.1103/PHYSREVB.75.052410
N. J. Laurita, J. Deisenhofer, LiDong Pan, C. M. Morris, M. Schmidt, M. Johnsson, V. Tsurkan, A. Loidl, N. P. Armitage, Singlet-Triplet Excitations and Long-Range Entanglement in the Spin-Orbital Liquid Candidate FeSc 2 S 4 Physical Review Letters. ,vol. 114, pp. 207201- ,(2015) , 10.1103/PHYSREVLETT.114.207201
G. Chen, M. Hermele, L. Radzihovsky, Frustrated quantum critical theory of putative spin-liquid phenomenology in 6H-B-Ba(3)NiSb(2)O(9). Physical Review Letters. ,vol. 109, pp. 016402- 016402 ,(2012) , 10.1103/PHYSREVLETT.109.016402
Hiroshi Murakawa, Yoshinori Onose, Kenya Ohgushi, Shintaro Ishiwata, Yoshinori Tokura, Generation of Electric Polarization with Rotating Magnetic Field in Helimagnet ZnCr2Se4 Journal of the Physical Society of Japan. ,vol. 77, pp. 043709- ,(2008) , 10.1143/JPSJ.77.043709
A. A. Burkov, M. D. Hook, Leon Balents, Topological nodal semimetals Physical Review B. ,vol. 84, pp. 235126- ,(2011) , 10.1103/PHYSREVB.84.235126