Novel insight into VOC removal performance of photocatalytic oxidation reactors

作者: Jinhan Mo , Yinping Zhang , Rui Yang

DOI: 10.1111/J.1600-0668.2005.00374.X

关键词:

摘要: A general model has been developed for analyzing the removal of volatile organic compounds (VOCs) by photocatalytic oxidation (PCO) reactors, taking into consideration (surface) reaction and con- vective mass transfer coefficients including allowance their spatial depend- ence. On this basis, a novel insight VOC performance PCO reactors is presented. The key parameter evaluating reactor number unit (NTUm), which shown to be simple linear product three dimensionless parameters: ratio area cross-sectional flow channel (A*), Stanton (Stm), effectiveness (g). A* represents geometric structural characteristic reactor. Stm shows synergistic degree alignment between fluid fields, reflects convective rate g, describes relative intensity rate. By using relationship parameters, influence various factors on performance, bottleneck improving design can determined. Three examples are used illustrate application our proposed model. It found that honeycomb type reactor, while light-in-tube With six fins fractional conversion increases about 70% one without any fins.

参考文章(19)
L. Mølhave, The sick buildings and other buildings with indoor climate problems Environment International. ,vol. 15, pp. 65- 74 ,(1989) , 10.1016/0160-4120(89)90011-1
Timothy N. Obee, Photooxidation of Sub-Parts-per-Million Toluene and Formaldehyde Levels on Titania Using a Glass-Plate Reactor Environmental Science & Technology. ,vol. 30, pp. 3578- 3584 ,(1996) , 10.1021/ES9602713
Yinping Zhang, Rui Yang, Rongyi Zhao, A model for analyzing the performance of photocatalytic air cleaner in removing volatile organic compounds Atmospheric Environment. ,vol. 37, pp. 3395- 3399 ,(2003) , 10.1016/S1352-2310(03)00357-1
Young Min Kim, Stuart Harrad, Roy M. Harrison, Concentrations and sources of VOCs in urban domestic and public microenvironments. Environmental Science & Technology. ,vol. 35, pp. 997- 1004 ,(2001) , 10.1021/ES000192Y
William J. Fisk, Arthur H. Rosenfeld, Estimates of Improved Productivity and Health from Better Indoor Environments Indoor Air. ,vol. 7, pp. 158- 172 ,(1997) , 10.1111/J.1600-0668.1997.T01-1-00002.X
Roman Meininghaus, Tunga Salthammer, Helmut Knöppel, Interaction of volatile organic compounds with indoor materials—a small-scale screening method Atmospheric Environment. ,vol. 33, pp. 2395- 2401 ,(1999) , 10.1016/S1352-2310(98)00367-7
Rui Yang, Yin-Ping Zhang, Rong-Yi Zhao, An improved model for analyzing the performance of photocatalytic oxidation reactors in removing volatile organic compounds and its application. Journal of The Air & Waste Management Association. ,vol. 54, pp. 1516- 1524 ,(2004) , 10.1080/10473289.2004.10471016
Md. Moazzem Hossain, Gregory B. Raupp, Steven O. Hay, Timothy N. Obee, Three‐dimensional developing flow model for photocatalytic monolith reactors Aiche Journal. ,vol. 45, pp. 1309- 1321 ,(1999) , 10.1002/AIC.690450615