Long-range transport of biomass burning emissions based on organic molecular markers and carbonaceous thermal distribution.

作者: Min-Suk Bae , Ju-Seon Shin , Kwang-Yul Lee , Kwon-Ho Lee , Young J. Kim

DOI: 10.1016/J.SCITOTENV.2013.06.096

关键词:

摘要: Semi-continuous organic carbon (OC), elemental (EC), and molecular markers were analyzed using the thermal optical transmittance method at Gosan supersite (on Jeju Island, Korea), which has been widely used as a regional background site for East Asia. The Carbonaceous Thermal Distribution (CTD) method, can provide detailed signature characteristics relative to analytical temperature, was improve fractionation of method. Ground-based measurements conducted from October 25 November 5, 2010. During sampling period, one high OC concentration event two characteristic periods observed. Considering distribution patterns, relationship between EC black (BC) by measurements, backward trajectories, aerosol thickness, PM10 concentrations 316 PM-network sites that operated Ministry Environment in Korea, markers, such levoglucosan, PAHs, acids, we concluded influenced long-range transport biomass burning emissions. This study discusses CTD analysis with marker concentrations, extracts interprets additional fractions semi-continuous data set, provides knowledge regarding origin sources their behaviors.

参考文章(52)
M. Radzi bin Abas, Daniel R. Oros, B.R.T. Simoneit, Biomass burning as the main source of organic aerosol particulate matter in Malaysia during haze episodes. Chemosphere. ,vol. 55, pp. 1089- 1095 ,(2004) , 10.1016/J.CHEMOSPHERE.2004.02.002
Min-Suk Bae, James J. Schauer, Jeffery T. DeMinter, Jay R. Turner, Hourly and daily patterns of particle-phase organic and elemental carbon concentrations in the urban atmosphere. Journal of The Air & Waste Management Association. ,vol. 54, pp. 823- 833 ,(2004) , 10.1080/10473289.2004.10470957
Cheol-Heon Jeong, Philip K. Hopke, Eugene Kim, Doh-Won Lee, The comparison between thermal-optical transmittance elemental carbon and Aethalometer black carbon measured at multiple monitoring sites Atmospheric Environment. ,vol. 38, pp. 5193- 5204 ,(2004) , 10.1016/J.ATMOSENV.2004.02.065
Joyce M. Harris, Jonathan D. W. Kahl, Analysis of 10-day isentropic flow patterns for Barrow, Alaska: 1985–1992 Journal of Geophysical Research. ,vol. 99, pp. 25845- 25855 ,(1994) , 10.1029/94JD02324
Oscar Peralta, Darrel Baumgardner, Graciela B. Raga, Spectrothermography of carbonaceous particles Journal of Atmospheric Chemistry. ,vol. 57, pp. 153- 169 ,(2007) , 10.1007/S10874-007-9070-1
R.M. Duvall, B.J. Majestic, M.M. Shafer, P.Y. Chuang, B.R.T. Simoneit, J.J. Schauer, The water-soluble fraction of carbon, sulfur, and crustal elements in Asian aerosols and Asian soils Atmospheric Environment. ,vol. 42, pp. 5872- 5884 ,(2008) , 10.1016/J.ATMOSENV.2008.03.028
Oliver V. Rattigan, H. Dirk Felton, Min-Suk Bae, James J. Schwab, Kenneth L. Demerjian, Multi-year hourly PM2.5 carbon measurements in New York: Diurnal, day of week and seasonal patterns Atmospheric Environment. ,vol. 44, pp. 2043- 2053 ,(2010) , 10.1016/J.ATMOSENV.2010.01.019
Timothy S. Bates, Barry J. Huebert, John L. Gras, F. Brian Griffiths, Philip A. Durkee, International Global Atmospheric Chemistry (IGAC) Project's First Aerosol Characterization Experiment (ACE 1): Overview Journal of Geophysical Research. ,vol. 103, pp. 16297- 16318 ,(1998) , 10.1029/97JD03741
Philip K. Hopke, Contemporary threats and air pollution Atmospheric Environment. ,vol. 43, pp. 87- 93 ,(2009) , 10.1016/J.ATMOSENV.2008.09.053