The nature of the Raman damping constant and its effect upon resonant light scattering from molecular systems in the weak field limit

作者: J.M. Friedman

DOI: 10.1016/0038-1098(79)90993-1

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摘要: Abstract With the use of a time dependent tetradic operator scattering formalism, comparison is made between resonant light (RLS) generated by monochromatic and pulsed excitations. This reveals that Raman damping constant reciprocal total dephasing associated with ensembles. A discussion given effect lifetime both excited intermediate state (T1) phase relationship pairs contributing states (T∗2) upon coherent incoherent makeup RLS. The question resonance versus fluorescence again reexamined.

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