Highly Efficient Water Splitting into H2 and O2 over Lanthanum-Doped NaTaO3 Photocatalysts with High Crystallinity and Surface Nanostructure

作者: Hideki Kato , Kiyotaka Asakura , Akihiko Kudo

DOI: 10.1021/JA027751G

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摘要: NiO-loaded NaTaO3 doped with lanthanum showed a high photocatalytic activity for water splitting into H2 and O2 in a stoichiometric amount under UV irradiation. The photocatalytic activity of NiO-loaded NaTaO3 doped with lanthanum was 9 times higher than that of nondoped NiO-loaded NaTaO3. The maximum apparent quantum yield of the NiO/NaTaO3: La photocatalyst was 56% at 270 nm. The factors affecting the highly efficient photocatalytic water splitting were examined by using various characterization techniques. Electron …

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