Transmutation of minor actinides in the pressurized water reactors

作者: Bin Liu , Kai Wang , Jing Tu , Fang Liu , Liming Huang

DOI: 10.1016/J.ANUCENE.2013.09.042

关键词:

摘要: We study the effects of adding MA nuclides to PWR core and nuclide transmutation rate in PWRs. Our calculation results show that even 1% homogeneous addition nuclear fuel can reduce keff PWRs drastically. The uniform distribution uranium dioxide also affect lifetime a loading. Calculation indicate reactivity mismatch control difficulties spatial self-shielding heterogeneous distributions avoid initial drop significantly, be overcome. During 300-day-exposure 14.8% Pu-238 7.7% Pu-239 are created, this explains at least 22.5% transmute plutonium isotopes during by various processes. may incinerate plutonium-239 plutonium-238 subsequent MOX loading Alternatively, we use created fabricate batteries. mainly transmuted from neptunium-237 PWRs, constitutes 56.2% total minor actinides depleted majority commercial reactors operation world if get their power generating, inventory high level long-lived radioactive will greatly reduced. Our actually act as burnable poisons materials used partially substitute for or concentration boric acid coolant increase negative temperature coefficient This is distinct advantage characteristics flux thermal compared research.

参考文章(20)
Samuel Glasstone, Alexander Sesonske, Nuclear Reactor Engineering ,(1955)
A Herrera-Martínez, Transmutation of nuclear waste in accelerator-driven systems University of Cambridge. ,(2004)
W. S. Yang, Y. Kim, R. N. Hill, T. A. Taiwo, H. S. Khalil, Long-Lived Fission Product Transmutation Studies Nuclear Science and Engineering. ,vol. 146, pp. 291- 318 ,(2004) , 10.13182/NSE04-A2411
James J. Duderstadt, Louis J. Hamilton, Nuclear reactor analysis ,(1976)
Toshikazu Takeda, Kenji Yokoyama, Study on neutron spectrum for effective transmutation of minor actinides in thermal reactors Annals of Nuclear Energy. ,vol. 24, pp. 705- 719 ,(1997) , 10.1016/S0306-4549(96)00035-7
Adonai Herrera-Martínez, Yacine Kadi, Geoffrey Parks, Marcus Dahlfors, Transmutation of nuclear waste in accelerator-driven systems: Fast spectrum Annals of Nuclear Energy. ,vol. 34, pp. 550- 563 ,(2007) , 10.1016/J.ANUCENE.2007.02.008
Vladimir Artisyuk, Masaki Saito, Alexey Stankovsky, Challenge of transmutation of long-lived nuclides Progress in Nuclear Energy. ,vol. 47, pp. 327- 338 ,(2005) , 10.1016/J.PNUCENE.2005.05.031
Tomohiko IWASAKI, Naohiro HIRAKAWA, Neutron Economy of Transmutation of TRU in Thermal and Fast Neutron Fields Journal of Nuclear Science and Technology. ,vol. 31, pp. 1255- 1264 ,(1994) , 10.1080/18811248.1994.9735288
Bin Liu, Wenchao Hu, Kai Wang, Liming Huang, Xiaoping Ouyang, Jing Tu, Yangni Zhu, Transmutation of MA in the high flux thermal reactor Journal of Nuclear Materials. ,vol. 437, pp. 95- 101 ,(2013) , 10.1016/J.JNUCMAT.2013.01.348
Bin Liu, Xuefeng Lv, Wei Zhao, Kai Wang, Jing Tu, Xiaoping Ouyang, The comparison of MCNP perturbation technique with MCNP difference method in critical calculation Nuclear Engineering and Design. ,vol. 240, pp. 2005- 2010 ,(2010) , 10.1016/J.NUCENGDES.2010.04.022