Chapter 5 Multidimensional Electronic and Vibrational Spectroscopy: An Ultrafast Probe of Molecular Relaxation and Reaction Dynamics
作者： Jennifer P. Ogilvie , Kevin J. Kubarych
DOI: 10.1016/S1049-250X(09)57005-X
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摘要: Abstract Multidimensional optical spectroscopy in the visible and infrared is a rapidly developing technique enabling direct observation of complex dynamics molecules environments such as liquids proteins. Measuring correlation between excited detected frequencies with sub‐picosecond resolution has enabled long‐standing problems energy transfer photosynthesis life‐sustaining structural rearrangements liquid water. This chapter aims to provide bridge concepts familiar AMO physics community how those ideas experimental methods are applied condensed phase molecular spectroscopy. We outline technical challenges these powerful while considering few examples experiments that showcase unique perspective offered by 2D electronic vibrational
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