A new kinetic approach to modeling water-rock interaction: The role of nucleation, precursors, and Ostwald ripening
作者： Carl I. Steefel , Philippe Van Cappellen
DOI: 10.1016/0016-7037(90)90003-4
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摘要: A new approach to water-rock interaction is developed which replaces the assumption of partial equilibrium with a complete calculation of the rates at which minerals form and dissolve. The evolution of reaction-flow systems towards equilibrium with respect to secondary phases is examined in terms of the important processes which generate and modify reactive surface areas of minerals: heterogeneous nucleation, crystal growth, dissolution, and crystal ripening. The widespread occurrence in surficial environments of …
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