Atmospheric concentrations of persistent organic pollutants over the Pacific Ocean near southern Taiwan and the northern Philippines.
作者： How-Ran Chao , Ding-Yan Lin , Kuang-Yu Chen , Yan-Yu Gou , Tsyr-Huei Chiou
DOI: 10.1016/J.SCITOTENV.2014.03.017
关键词: Pollutant 、 Polybrominated Biphenyls 、 Polychlorinated diphenyl ethers 、 Polybrominated diphenyl ethers 、 Atmosphere 、 Congener 、 Environmental chemistry 、 Pacific ocean 、 Southern taiwan 、 Environmental science
摘要: This study investigates the atmospheric occurrence of persistent organic pollutants (POPs) over Pacific Ocean near southern Taiwan and northern Philippines. We determined sixty-six compounds, including polychlorinated dibenzo-p-dioxins dibenzofurans (PCDD/Fs), dioxin-like biphenyls (DLPCBs), polybrominated diphenyl ethers (PBDEs), as well (PCDEs), (PBDD/Fs), (PBBs), in air samples simultaneously collected from offshore oceanic atmosphere (n=6) a rural area (n=2). calculated World Health Organization 2005 toxic equivalency levels (WHO2005-TEQ), for total POPs, PCDD/Fs, DLPCBs, PBDD/Fs, being 0.00612 pg WHO2005-TEQ/m(3) 0.0138 ocean land, respectively. found unexpected lower averaged PBDE concentrations (15.9 pg/m(3)) than (31.1 due to higher BDE209 congener, although difference was not statistically significant. have compared reported our field results with previously published datasets global oceans, which suggest PCBs PBDEs are dominant chemical contaminants among these halogenated POPs (e.g. Σdi-hepta could be range 0.09-48.7 8.07-94.0 pg/m(3), respectively, dataset). However, there still very few investigations on PCDEs PBBs data sums earlier studies. Finally, we point out that originated or continental East Asia easily reach remote sites via transport.
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sci-hub.se 参考文章(51)
Ping-Chi Hsu, Yueliang Leon Guo, Derek R. Smith, Yu-Sheng Lin, Li-Ho Tseng, Chia-Wei Lee, Jenq-Renn Chen, Airborne persistent organic pollutants and male reproductive health. Aerosol and Air Quality Research. ,vol. 14, pp. 1292- 1298 ,(2014) , 10.4209/AAQR.2013.03.0066
Lin-Chi Wang, Cheng-Hsien Tsai, Guo-Ping Chang-Chien, Chung-Hsien Hung, Characterization of polybrominated dibenzo-p-dioxins and dibenzofurans in different atmospheric environments. Environmental Science & Technology. ,vol. 42, pp. 75- 80 ,(2008) , 10.1021/ES071924Q
H.-R. Chao, S.-L. Wang, L.-Y. Lin, W.-J. Lee, O. Päpke, Placental transfer of polychlorinated dibenzo-p-dioxins, dibenzofurans, and biphenyls in Taiwanese mothers in relation to menstrual cycle characteristics. Food and Chemical Toxicology. ,vol. 45, pp. 259- 265 ,(2007) , 10.1016/J.FCT.2006.07.032
Rosalinda Gioia, Jun Li, Jasmin Schuster, Yanlin Zhang, Gan Zhang, Xiangdong Li, Baruch Spiro, Ravinder S Bhatia, Jordi Dachs, Kevin C Jones, None, Factors Affecting the Occurrence and Transport of Atmospheric Organochlorines in the China Sea and the Northern Indian and South East Atlantic Oceans Environmental Science & Technology. ,vol. 46, pp. 10012- 10021 ,(2012) , 10.1021/ES302037T
Lin-Chi Wang, Hsing-Cheng Hsi, Ya-Fen Wang, Sheng-Lun Lin, Guo-Ping Chang-Chien, Distribution of polybrominated diphenyl ethers (PBDEs) and polybrominated dibenzo-p-dioxins and dibenzofurans (PBDD/Fs) in municipal solid waste incinerators. Environmental Pollution. ,vol. 158, pp. 1595- 1602 ,(2010) , 10.1016/J.ENVPOL.2009.12.016
Axel Möller, Zhiyong Xie, Minghong Cai, Renate Sturm, Ralf Ebinghaus, Brominated flame retardants and dechlorane plus in the marine atmosphere from Southeast Asia toward Antarctica. Environmental Science & Technology. ,vol. 46, pp. 3141- 3148 ,(2012) , 10.1021/ES300138Q
Lin-Chi Wang, Wen-Jhy Lee, Wei-Shan Lee, Guo-Ping Chang-Chien, Polybrominated diphenyl ethers in various atmospheric environments of Taiwan: their levels, source identification and influence of combustion sources. Chemosphere. ,vol. 84, pp. 936- 942 ,(2011) , 10.1016/J.CHEMOSPHERE.2011.06.008
Aullya Ardhini Artha, Edward Ming-Yang Wu, Lin-Chi Wang, Chi-Hsuan Chen, Guo-Ping Chang-Chien, Thermal Formation of Polybrominated Diphenyl Ethers in Raw and Water-Washed Fly Ash Aerosol and Air Quality Research. ,vol. 11, pp. 393- 400 ,(2011) , 10.4209/AAQR.2011.04.0039
Rainer Lohmann, Jana Klanova, Petr Kukucka, Shifra Yonis, Kevyn Bollinger, PCBs and OCPs on a East-to-West Transect: The Importance of Major Currents and Net Volatilization for PCBs in the Atlantic Ocean Environmental Science & Technology. ,vol. 46, pp. 10471- 10479 ,(2012) , 10.1021/ES203459E
Urs Schenker, Fabian Soltermann, Martin Scheringer, Konrad Hungerbühler, Modeling the environmental fate of polybrominated diphenyl ethers (PBDEs): the importance of photolysis for the formation of lighter PBDEs. Environmental Science & Technology. ,vol. 42, pp. 9244- 9249 ,(2008) , 10.1021/ES801042N