Giant Rashba splitting in graphene due to hybridization with gold

作者: D. Marchenko , A. Varykhalov , M.R. Scholz , G. Bihlmayer , E.I. Rashba

DOI: 10.1038/NCOMMS2227

关键词: CouplingCondensed matter physicsFermi energyAb initioSpintronicsSpin (physics)X-ray photoelectron spectroscopyElectronMaterials scienceGraphene

摘要: Graphene in spintronics is predominantly considered for spin current leads of high performance due to weak intrinsic spin–orbit coupling of the graphene π electrons. Externally induced large spin–orbit coupling opens the possibility of using graphene in active elements of spintronic devices such as the Das-Datta spin field-effect transistor. Here we show that Au intercalation at the graphene–Ni interface creates a giant spin–orbit splitting (~ 100 meV) of the graphene Dirac cone up to the Fermi energy. Photoelectron …

参考文章(40)
Chun Li, A. J. Freeman, H. J. F. Jansen, C. L. Fu, Magnetic anisotropy in low-dimensional ferromagnetic systems: Fe monolayers on Ag(001), Au(001), and Pd(001) substrates. Physical Review B. ,vol. 42, pp. 5433- 5442 ,(1990) , 10.1103/PHYSREVB.42.5433
A. Varykhalov, M. R. Scholz, Timur K. Kim, O. Rader, Effect of noble-metal contacts on doping and band gap of graphene Physical Review B. ,vol. 82, pp. 121101- ,(2010) , 10.1103/PHYSREVB.82.121101
John P. Perdew, Kieron Burke, Matthias Ernzerhof, Generalized Gradient Approximation Made Simple Physical Review Letters. ,vol. 77, pp. 3865- 3868 ,(1996) , 10.1103/PHYSREVLETT.77.3865
S. LaShell, B. A. McDougall, E. Jensen, Spin Splitting of an Au(111) Surface State Band Observed with Angle Resolved Photoelectron Spectroscopy. Physical Review Letters. ,vol. 77, pp. 3419- 3422 ,(1996) , 10.1103/PHYSREVLETT.77.3419
Y. G. Semenov, K. W. Kim, J. M. Zavada, Spin field effect transistor with a graphene channel Applied Physics Letters. ,vol. 91, pp. 153105- ,(2007) , 10.1063/1.2798596
J. Jacobsen, L. Pleth Nielsen, F. Besenbacher, I. Stensgaard, E. Lægsgaard, T. Rasmussen, K. W. Jacobsen, J. K. Nørskov, Atomic-scale determination of misfit dislocation loops at metal-metal interfaces. Physical Review Letters. ,vol. 75, pp. 489- 492 ,(1995) , 10.1103/PHYSREVLETT.75.489
F. Reinert, G. Nicolay, S. Schmidt, D. Ehm, S. Hüfner, Direct measurements of the L -gap surface states on the (111) face of noble metals by photoelectron spectroscopy Physical Review B. ,vol. 63, pp. 115415- ,(2001) , 10.1103/PHYSREVB.63.115415
Aaron Bostwick, Taisuke Ohta, Thomas Seyller, Karsten Horn, Eli Rotenberg, Quasiparticle dynamics in graphene Nature Physics. ,vol. 3, pp. 36- 40 ,(2007) , 10.1038/NPHYS477
D. Huertas-Hernando, F. Guinea, Arne Brataas, Spin-orbit-mediated spin relaxation in graphene. Physical Review Letters. ,vol. 103, pp. 146801- ,(2009) , 10.1103/PHYSREVLETT.103.146801
P. Stoppmanns, B. Heidemann, N. Irmer, N. Müller, B. Vogt, B. Schmiedeskamp, U. Heinzmann, E. Tamura, R. Feder, Au-induced surface state on Pt(111) revealed by spin-resolved photoemission with linearly polarized light. Physical Review Letters. ,vol. 66, pp. 2645- 2648 ,(1991) , 10.1103/PHYSREVLETT.66.2645