An investigation of the dosimetric and kinetic properties of sand using ESR and TL techniques.

作者: Canan Aydaş , Talat Aydın

DOI: 10.1016/J.APRADISO.2015.03.019

关键词: IrradiationElectron paramagnetic resonanceKinetic energyThermoluminescenceKineticsAnalytical chemistryActivation energyAnnealing (metallurgy)Absorbed doseChemistry

摘要: Abstract In this research, the general dosimetric and kinetic properties of sand from a beach in southern Turkey were investigated using electron spin resonance (ESR) thermoluminescence (TL) techniques. The ESR dose response curve presents linear behaviour range 250–1000 Gy followed by sublinear 2–8 kGy. Kinetic behaviors activation energy free radical also calculated data obtained annealing studies performed at four different temperatures (220, 240, 260 280 °C). value was as 1.47 eV. long-term fading signal room temperature turned out to be best described second-order decay function. presence measurable intensity even after storage period 90 days considered providing an opportunity estimation irradiated sample. Although TL glow natural (unirradiated) sample only has single broad peak 317 °C, peaks located ~115 °C, ~156 °C, ~231 °C ~308 °C their tends increased with absorbed dose. T m x − s t o p fitting results showed that least five ∼116 °C, 149 °C, 228 °C, 306 °C 360 °C. This result suggests apparently D may consist two or more overlapping peaks. According thermal temperature, intensities (23 °C 308 °C) found quite large 30 allows accurate measurement intensity. additive method, variable heating rate method (VHRM), used number peaks, parameters. study shows techniques could successfully investigate kinetics Furthermore, plus previous work done authors suggest could, techniques, suitable material for alternative measurement.

参考文章(35)
Reuven Chen, Stephen W S McKeever, THEORY OF THERMOLUMINESCENCE AND RELATED PHENOMENA ,(1997)
GM FERRAZ, Gilberto Marcon Ferraz, Gilberto M Ferraz, MI TEIXEIRA, L CALDAS, Sand for high-dose dosimetry using the EPR technique. Applied Radiation and Isotopes. ,vol. 62, pp. 359- 363 ,(2005) , 10.1016/J.APRADISO.2004.08.023
M. G. Jani, R. B. Bossoli, L. E. Halliburton, Further characterization of theE1′center in crystalline SiO2 Physical Review B. ,vol. 27, pp. 2285- 2293 ,(1983) , 10.1103/PHYSREVB.27.2285
F.O. Ogundare, M.L. Chithambo, E.O. Oniya, Anomalous behaviour of thermoluminescence from quartz: A case of glow peaks from a Nigerian quartz Radiation Measurements. ,vol. 41, pp. 549- 553 ,(2006) , 10.1016/J.RADMEAS.2006.03.001
Huang Pei-Hua, Jin Si-Zhao, Peng Zhi-Cheng, Liang Ren-Yu, Quan Yu-cai, Wang Zhao-Rong, ESR dating and trapped electrons lifetime of quartz grains in loess of China Quaternary Science Reviews. ,vol. 7, pp. 533- 536 ,(1988) , 10.1016/0277-3791(88)90058-3
Canan Aydaş, Birol Engin, Talat Aydın, Radiation-induced signals of gypsum crystals analysed by ESR and TL techniques applied to dating Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms. ,vol. 269, pp. 417- 424 ,(2011) , 10.1016/J.NIMB.2010.12.074
A Necmeddin Yazici, Mustafa Topaksu, The analysis of thermoluminescence glow peaks of unannealed synthetic quartz Journal of Physics D. ,vol. 36, pp. 620- 627 ,(2003) , 10.1088/0022-3727/36/6/303
S.G Vaijapurkar, R Raman, P.K Bhatnagar, Sand—a high gamma dose thermoluminescence dosimeter Radiation Measurements. ,vol. 29, pp. 223- 226 ,(1998) , 10.1016/S1350-4487(97)00229-1