Nonlinear optical properties of the fullerenes C60 and C70 at 1.064 microm.
作者： J. R. Lindle , R. G. S. Pong , F. J. Bartoli , Z. H. Kafafi
关键词: Fullerene 、 Four-wave mixing 、 Laser 、 Molecular physics 、 Grating 、 Transmittance 、 Nonlinear optics 、 Materials science 、 Optics 、 Absorption (electromagnetic radiation) 、 Absorption spectroscopy
摘要: Time-resolved degenerate-four-wave-mixing experiments were conducted on films of pure C 60 and 70 using a 35-ps laser at 1.064 μm. The fullerenes exhibit two-photon resonantly enhanced third-order optical response that is primarily laser-pulse-limited. At high intensities, fifth-order component to the nonlinear signal observed attributed excited-state transient grating. large absorption coefficients measured for μm by transmittance are consistent with this assignment
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sci-hub.se 参考文章(28)
H. W. Kroto, J. R. Heath, S. C. O’Brien, R. F. Curl, R. E. Smalley, C 60 : Buckminsterfullerene Nature. ,vol. 318, pp. 162- 163 ,(1985) , 10.1038/318162A0
W. Krätschmer, Lowell D. Lamb, K. Fostiropoulos, Donald R. Huffman, Solid C60: a new form of carbon Nature. ,vol. 347, pp. 354- 358 ,(1990) , 10.1038/347354A0
Z.H. Kafafi, J.R. Lindle, R.G.S. Pong, F.J. Bartoli, L.J. Lingg, J. Milliken, Off-resonant nonlinear optical properties of C60 studied by degenerate four-wave mixing Chemical Physics Letters. ,vol. 188, pp. 492- 496 ,(1992) , 10.1016/0009-2614(92)80854-5
Ying Wang, Lap Tak Cheng, Nonlinear optical properties of fullerenes and charge-transfer complexes of fullerenes The Journal of Physical Chemistry. ,vol. 96, pp. 1530- 1532 ,(1992) , 10.1021/J100183A007
W. J. Blau, H. J. Byrne, D. J. Cardin, T. J. Dennis, J. P. Hare, H. W. Kroto, R. Taylor, D. R. M. Walton, Large infrared nonlinear optical response ofC60 Physical Review Letters. ,vol. 67, pp. 1423- 1425 ,(1991) , 10.1103/PHYSREVLETT.67.1423
R. J. Knize, J. P. Partanen, Comment on ‘‘Large infrared nonlinear optical response ofC60’’ Physical Review Letters. ,vol. 68, pp. 2704- 2704 ,(1992) , 10.1103/PHYSREVLETT.68.2704
Z. H. Kafafi, F. J. Bartoli, J. R. Lindle, R. G. S. Pong, Comment on ‘‘Large infrared nonlinear optical response ofC60’’ Physical Review Letters. ,vol. 68, pp. 2705- 2705 ,(1992) , 10.1103/PHYSREVLETT.68.2705
Lee W. Tutt, Alan Kost, Optical limiting performance of C60 and C70 solutions Nature. ,vol. 356, pp. 225- 226 ,(1992) , 10.1038/356225A0
Hajime Hoshi, Naoki Nakamura, Yusei Maruyama, Takashi Nakagawa, Shinzo Suzuki, Haruo Shiromaru, Yohji Achiba, Optical Second- and Third-Harmonic Generations in C60 Film Japanese Journal of Applied Physics. ,vol. 30, ,(1991) , 10.1143/JJAP.30.L1397
Jeffrey S. Meth, Herman Vanherzeele, Ying Wang, Dispersion of the third-order optical nonlinearity of C60. A third-harmonic generation study Chemical Physics Letters. ,vol. 197, pp. 26- 31 ,(1992) , 10.1016/0009-2614(92)86016-B