Measurement of NOx Fluxes from a Tall Tower in Central London, UK and Comparison with Emissions Inventories
作者： James D Lee , Carole Helfter , Ruth M Purvis , Sean D Beevers , David C Carslaw
DOI: 10.1021/ES5049072
关键词: Tower 、 Airflow 、 Eddy covariance 、 Atmospheric emissions 、 Time resolution 、 Flux (metallurgy) 、 Meteorology 、 NOx 、 Emission inventory
摘要: Direct measurements of NOx concentration and flux were made from a tall tower in central London, UK as part the Clean Air for London (ClearfLo) project. Fast time resolution (10 Hz) NO NO2 concentrations measured combined with fast vertical wind to provide top-down estimates using eddy covariance technique. Measured fluxes usually positive ranged close zero at night 2000–8000 ng m–2 s–1 during day. Peak observed morning, coincident maximum traffic flow. Measurements have been scaled compared National Atmospheric Emissions Inventory (NAEI) estimate emission measurement footprint. The are on average 80% higher than NAEI inventory all London. Observations westerly airflow (from parts where is smaller fraction source) showed better agreement inventory. observations sug...
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Thomas Foken, Mathias Göockede, Matthias Mauder, Larry Mahrt, Brian Amiro, William Munger, Post-Field Data Quality Control Handbook of Micrometeorology. pp. 181- 208 ,(2004) , 10.1007/1-4020-2265-4_9
William Massman, Xuhui Lee, Beverly Law, Handbook of micrometeorology : a guide for surface flux measurement and analysis Kluwer Academic. ,(2004)
RG Derwent, DR Middleton, RA Field, ME Goldstone, JN Lester, R Perry, Analysis and interpretation of air quality data from an urban roadside location in Central London over the period from July 1991 to July 1992 Atmospheric Environment. ,vol. 29, pp. 923- 946 ,(1995) , 10.1016/1352-2310(94)00219-B
Robert Kormann, Franz X. Meixner, An Analytical Footprint Model For Non-Neutral Stratification Boundary-Layer Meteorology. ,vol. 99, pp. 207- 224 ,(2001) , 10.1023/A:1018991015119
Peter S. Bakwin, Steven C. Wofsy, Song-Miao Fan, David R. Fitzjarrald, Measurements of NO(x) and NO(y) concentrations and fluxes over Arctic tundra Journal of Geophysical Research. ,vol. 97, pp. 16545- 16557 ,(1992) , 10.1029/91JD00929
Ilana B. Pollack, Brian M. Lerner, Thomas B. Ryerson, Evaluation of ultraviolet light-emitting diodes for detection of atmospheric NO2 by photolysis - chemiluminescence Journal of Atmospheric Chemistry. ,vol. 65, pp. 111- 125 ,(2010) , 10.1007/S10874-011-9184-3
Qi Ying, Jin Lu, Paul Allen, Paul Livingstone, Ajith Kaduwela, Michael Kleeman, Modeling air quality during the California Regional PM10/PM2.5 Air Quality Study (CRPAQS) using the UCD/CIT source-oriented air quality model -Part I. Base case model results Atmospheric Environment. ,vol. 42, pp. 8954- 8966 ,(2008) , 10.1016/J.ATMOSENV.2008.05.064
J. D. Lee, S. J. Moller, K. A. Read, A. C. Lewis, L. Mendes, L. J. Carpenter, Year‐round measurements of nitrogen oxides and ozone in the tropical North Atlantic marine boundary layer Journal of Geophysical Research. ,vol. 114, ,(2009) , 10.1029/2009JD011878
David C. Carslaw, Sean D. Beevers, Investigating the potential importance of primary NO2 emissions in a street canyon Atmospheric Environment. ,vol. 38, pp. 3585- 3594 ,(2004) , 10.1016/J.ATMOSENV.2004.03.041
R.E Honrath, Y Lu, M.C Peterson, J.E Dibb, M.A Arsenault, N.J Cullen, K Steffen, Vertical fluxes of NOx, HONO, and HNO3 above the snowpack at Summit, Greenland Atmospheric Environment. ,vol. 36, pp. 2629- 2640 ,(2002) , 10.1016/S1352-2310(02)00132-2