Slowing down of the global accumulation of atmospheric methane during the 1980s

作者: L. P. Steele , E. J. Dlugokencky , P. M. Lang , P. P. Tans , R. C. Martin

DOI: 10.1038/358313A0

关键词: Fossil fuelTroposphereMixing ratioAtmospheric sciencesChemistryAtmospheric methaneMeteorologyLatitudeAtmosphereMethaneEarth's energy budget

摘要: MEASUREMENTS of methane in modern air1–8 and air trapped ice cores9–12 have shown convincingly that the abundance atmospheric has been rising since Industrial Revolution. This is a matter concern because important role determining radiative balance chemical composition atmosphere13. The causes this increase not identified unambiguously uncertainties our understanding global budget methane14 how it changing with time. Here we report on measurements from an extensive network flask sampling sites, which reveal that, although continues to accumulate atmosphere, there substantial slowing accumulation rate between 1983 1990. If deceleration steadily, concentrations will reach maximum around year 2006. Our results hint changes emissions latitude band 30–90° N may be particular significance trend.

参考文章(21)
D.M. Etheridge, G.I. Pearman, F. de Silva, Atmospheric trace-gas variations as revealed by air trapped in an ice core from Law Dome, Antarctica Annals of Glaciology. ,vol. 10, pp. 28- 33 ,(1988) , 10.1017/S0260305500004110
R. Prinn, D. Cunnold, P. Simmonds, F. Alyea, R. Boldi, A. Crawford, P. Fraser, D. Gutzler, D. Hartley, R. Rosen, R. Rasmussen, Global average concentration and trend for hydroxyl radicals deduced from ALE/GAGE trichloroethane (methyl chloroform) data for 1978–1990 Journal of Geophysical Research. ,vol. 97, pp. 2445- 2461 ,(1992) , 10.1029/91JD02755
Persi Diaconis, Bradley Efron, Computer-Intensive Methods in Statistics Scientific American. ,vol. 248, pp. 116- 130 ,(1983) , 10.1038/SCIENTIFICAMERICAN0583-116
P. J. Fraser, P. Hyson, R. A. Rasmussen, A. J. Crawford, M. A. K. Khalil, Methane, carbon monoxide and methylchloroform in the southern hemisphere Journal of Atmospheric Chemistry. ,vol. 4, pp. 3- 42 ,(1986) , 10.1007/BF00053771
D. R. BLAKE, F. S. ROWLAND, Continuing worldwide increase in tropospheric methane, 1978 to 1987. Science. ,vol. 239, pp. 1129- 1131 ,(1988) , 10.1126/SCIENCE.239.4844.1129
B. STAUFFER, G. FISCHER, A. NEFTEL, H. OESCHGER, Increase of Atmospheric Methane Recorded in Antarctic Ice Core Science. ,vol. 229, pp. 1386- 1388 ,(1985) , 10.1126/SCIENCE.229.4720.1386
L. P. Steele, P. J. Fraser, R. A. Rasmussen, M. A. K. Khalil, T. J. Conway, A. J. Crawford, R. H. Gammon, K. A. Masarie, K. W. Thoning, The global distribution of methane in the troposphere Journal of Atmospheric Chemistry. ,vol. 5, pp. 125- 171 ,(1987) , 10.1007/978-94-009-3909-7_21
Donald R. Blake, F. Sherwood Rowland, World-wide increase in tropospheric methane, 1978–1983 Journal of Atmospheric Chemistry. ,vol. 4, pp. 43- 62 ,(1986) , 10.1007/BF00053772
Ghanshyam L. Vaghjiani, A. R. Ravishankara, New Measurement of the rate coefficient for the reaction of OH with methane. Nature. ,vol. 350, pp. 406- 409 ,(1991) , 10.1038/350406A0
R. S. Bradley, H. F. Diaz, G. N. Kiladis, J. K. Eischeid, ENSO signal in continental temperature and precipitation records Nature. ,vol. 327, pp. 497- 501 ,(1987) , 10.1038/327497A0