Large-area spatially ordered arrays of gold nanoparticles directed by lithographically confined DNA origami.
作者： Albert M. Hung , Christine M. Micheel , Luisa D. Bozano , Lucas W. Osterbur , Greg M. Wallraff
关键词: Materials science 、 Nanoparticle 、 Nanobiotechnology 、 Molecular nanotechnology 、 Nanoscopic scale 、 Nanomaterials 、 Nanotechnology 、 Lithography 、 DNA origami 、 Colloidal gold
摘要: The development of nanoscale electronic and photonic devices will require a combination the high throughput lithographic patterning resolution chemical precision afforded by self-assembly. However, incorporation nanomaterials with dimensions less than 10 nm into functional has been hindered disparity between their size 100 feature sizes that can be routinely generated lithography. Biomolecules offer bridge two regimes, sub-10 dimensions, synthetic flexibility capability for self-recognition. Here, we report directed assembly 5-nm gold particles large-area, spatially ordered, two-dimensional arrays through site-selective deposition mesoscopic DNA origami onto lithographically patterned substrates precise binding nanocrystals to each structure. We show organization registry both within an individual template components on neighbouring origami, expanding generality this method towards many types patterns sizes.
nature.com
harvard.edu
sci-hub.se 参考文章(29)
Erik Winfree, Furong Liu, Lisa A. Wenzler, Nadrian C. Seeman, Design and self-assembly of two-dimensional DNA crystals Nature. ,vol. 394, pp. 539- 544 ,(1998) , 10.1038/28998
Yonghai Song, Zhuang Li, Zhiguo Liu, Gang Wei, Li Wang, Lanlan Sun, Cunlan Guo, Yujing Sun, Tao Yang, A Novel Strategy to Construct a Flat-Lying DNA Monolayer on a Mica Surface Journal of Physical Chemistry B. ,vol. 110, pp. 10792- 10798 ,(2006) , 10.1021/JP0564344
Shawn M. Douglas, Hendrik Dietz, Tim Liedl, Björn Högberg, Franziska Graf, William M. Shih, Self-assembly of DNA into nanoscale three-dimensional shapes Nature. ,vol. 459, pp. 414- 418 ,(2009) , 10.1038/NATURE08016
Chengde Mao, Weiqiong Sun, Nadrian C. Seeman, Assembly of Borromean rings from DNA Nature. ,vol. 386, pp. 137- 138 ,(1997) , 10.1038/386137B0
J. Sharma, R. Chhabra, A. Cheng, J. Brownell, Y. Liu, H. Yan, Control of Self-Assembly of DNA Tubules Through Integration of Gold Nanoparticles Science. ,vol. 323, pp. 112- 116 ,(2009) , 10.1126/SCIENCE.1165831
Dmytro Nykypanchuk, Mathew M. Maye, Daniel van der Lelie, Oleg Gang, DNA-guided crystallization of colloidal nanoparticles Nature. ,vol. 451, pp. 549- 552 ,(2008) , 10.1038/NATURE06560
Daniela Zanchet, Christine M. Micheel, Wolfgang J. Parak, Daniele Gerion, A. Paul Alivisatos, Electrophoretic Isolation of Discrete Au Nanocrystal/DNA Conjugates Nano Letters. ,vol. 1, pp. 32- 35 ,(2001) , 10.1021/NL005508E
Russell P Goodman, Iwan AT Schaap, Catherine F Tardin, Christoph M Erben, Richard M Berry, Christoph F Schmidt, Andrew J Turberfield, Rapid chiral assembly of rigid DNA building blocks for molecular nanofabrication. Science. ,vol. 310, pp. 1661- 1665 ,(2005) , 10.1126/SCIENCE.1120367
C. K. Choi, C. H. Margraves, K. D. Kihm, Examination of near-wall hindered Brownian diffusion of nanoparticles: Experimental comparison to theories by Brenner (1961) and Goldman et al. (1967) Physics of Fluids. ,vol. 19, pp. 103305- ,(2007) , 10.1063/1.2798811
Y. Weizmann, A. B. Braunschweig, O. I. Wilner, Z. Cheglakov, I. Willner, A polycatenated DNA scaffold for the one-step assembly of hierarchical nanostructures Proceedings of the National Academy of Sciences of the United States of America. ,vol. 105, pp. 5289- 5294 ,(2008) , 10.1073/PNAS.0800723105