Aerosol emissions by tropical forest and savanna biomass burning: Characteristic trace elements and fluxes

作者: F. Echalar , A. Gaudichet , H. Cachier , P. Artaxo

DOI: 10.1029/95GL03170

关键词: VegetationPotassiumAerosolTrace elementHydrologyBiogeochemical cycleAtmospheric sciencesDry seasonEnvironmental scienceEnrichment factorTropical savanna climate

摘要: Aerosol particles were collected during the dry season in amazonian forest and African Brazilian savannas. Sampling was performed inside plumes of vegetation fires local background atmosphere. Samples analysed for their elemental composition by Particle Induced X-Ray Emission (PIXE). Enrichment factors relative to calculated. Savanna fire aerosols are characterised enrichments elements like K, P, Cl, Zn, Br, whereas emissions enriched Si Ca. The unexpected low potassium enrichment factor could be due prevailing smoldering conditions, high values savanna associated with predominant flaming conditions. This result indicates that may considered a good tracer phase only. S, Ca, Mn, Br total particulate matter calculated fires. Our estimates annual zinc tropical indicate contribution this source should taken into account understand biogeochemical cycle these elements.

参考文章(15)
Yoram J. Kaufman, Alberto W. Setzer, Darold E. Ward, Rei A. Rasmussen, Characteristics of smoke emissions from biomass fires of the Amazon region - BASE-A experiment ,(1991)
Paul J Crutzen, Meinrat O Andreae, None, Biomass Burning in the Tropics: Impact on Atmospheric Chemistry and Biogeochemical Cycles Science. ,vol. 250, pp. 1669- 1678 ,(1990) , 10.1126/SCIENCE.250.4988.1669
Paulo Artaxo, Hedwig Storms, Frank Bruynseels, René Van Grieken, Willy Maenhaut, Composition and sources of aerosols from the Amazon Basin Journal of Geophysical Research. ,vol. 93, pp. 1605- 1615 ,(1988) , 10.1029/JD093ID02P01605
J. P. Lacaux, J. M. Brustet, R. Delmas, J. C. Menaut, L. Abbadie, B. Bonsang, H. Cachier, J. Baudet, M. O. Andreae, G. Helas, Biomass burning in the tropical savannas of Ivory Coast: An overview of the field experiment Fire of Savannas (FOS/DECAFE 91) Journal of Atmospheric Chemistry. ,vol. 22, pp. 195- 216 ,(1995) , 10.1007/BF00708189
H�l�ne Cachier, Catherine Liousse, Patrick Buat-Menard, Annie Gaudichet, Particulate content of savanna fire emissions Journal of Atmospheric Chemistry. ,vol. 22, pp. 123- 148 ,(1995) , 10.1007/BF00708185
M. O. Andreae, E. V. Browell, M. Garstang, G. L. Gregory, R. C. Harriss, G. F. Hill, D. J. Jacob, M. C. Pereira, G. W. Sachse, A. W. Setzer, P. L. Silva Dias, R. W. Talbot, A. L. Torres, S. C. Wofsy, Biomass-burning emissions and associated haze layers over Amazonia Journal of Geophysical Research. ,vol. 93, pp. 1509- 1527 ,(1988) , 10.1029/JD093ID02P01509
Jerome O. Nriagu, A global assessment of natural sources of atmospheric trace metals Nature. ,vol. 338, pp. 47- 49 ,(1989) , 10.1038/338047A0
A. Gaudichet, F. Echalar, B. Chatenet, J. P. Quisefit, G. Malingre, H. Cachier, P. Buat-Menard, P. Artaxo, W. Maenhaut, Trace-Elements in Tropical African Savanna Biomass Burning Aerosols. Journal of Atmospheric Chemistry. ,vol. 22, pp. 19- 39 ,(1995) , 10.1007/BF00708179
Jerome O. Nriagu, Jozef M. Pacyna, Quantitative assessment of worldwide contamination of air, water and soils by trace metals Nature. ,vol. 333, pp. 134- 139 ,(1988) , 10.1038/333134A0
Lance F. W. Lesack, Robert E. Hecky, John M. Melack, Transport of carbon, nitrogen, phosphorus, and major solutes in the Gambia River, West Africa1 Limnology and Oceanography. ,vol. 29, pp. 816- 830 ,(1984) , 10.4319/LO.1984.29.4.0816