作者: Atsushi Sugita , Kazuhiro Yanagi , Kazuyoshi Kuroyanagi , Hironori Takahashi , Shinichiro Aoshima
DOI: 10.1016/J.CPLETT.2003.10.115
关键词: Stimulated emission 、 Excited state 、 Ultrashort pulse 、 Ground state 、 Analytical chemistry 、 Femtosecond 、 Atomic physics 、 Relaxation (NMR) 、 Time-resolved spectroscopy 、 Absorption spectroscopy 、 Chemistry
摘要: Ultrafast photo-excitation dynamics of N-benzyl 2-methyl-4-nitroaniline was studied with femtosecond time-resolved absorption spectroscopy. The photo-induced spectrum found to consist three transient components different decay times. A 260 fs-decay time stimulated emission appeared during a geometrical relaxation from charge-transfer excited state geometrically relaxed state. following energy the completed within 680 fs. Third 2.6 ps reflected cooling process hot electrons in ground potential.