Dynamics of xenon, krypton, and methane monolayers in registry with graphite.
作者： T. M. Hakim , H. R. Glyde , S. T. Chui
关键词: Atomic physics 、 Anharmonicity 、 Brillouin zone 、 Materials science 、 Phase (matter) 、 Xenon 、 Krypton 、 Dispersion (chemistry) 、 Phonon 、 Dispersion relation
摘要: The self-consistent phonon (SCP) theory is used to study the dynamics of monolayers xenon, krypton, and methane adsorbed on graphite. Only ..sqrt..3 x solid phase considered. It shown that energies Xe are very similar those their floating counterparts, while interaction Kr CH/sub 4/ with graphite significantly affects dispersion curves. gap in curves at center Brillouin zone computed as a function temperature. At critical temperature, goes spontaneously zero transition from locked-in commensurate takes place. This appears describe well. A simple model compared full SCP calculations. one-phonon dynamic form factor, including cubic anharmonic term, lifetimes also evaluated for 4/.
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sci-hub.se 参考文章(51)
David R. Nelson, B. I. Halperin, Dislocation-mediated melting in two dimensions Physical Review B. ,vol. 19, pp. 2457- 2484 ,(1979) , 10.1103/PHYSREVB.19.2457
A. P. Young, Melting and the vector Coulomb gas in two dimensions Physical Review B. ,vol. 19, pp. 1855- 1866 ,(1979) , 10.1103/PHYSREVB.19.1855
S. T. Chui, Statistical mechanics of two-dimensional domain walls Physical Review B. ,vol. 23, pp. 5982- 5992 ,(1981) , 10.1103/PHYSREVB.23.5982
Farid F. Abraham, Computational statistical mechanics methodology, applications and supercomputing Advances in Physics. ,vol. 35, pp. 1- 111 ,(1986) , 10.1080/00018738600101851
H. Taub, K. Carneiro, J. K. Kjems, L. Passell, J. P. McTague, Neutron scattering study of 36 Ar monolayer films adsorbed on graphite Physical Review B. ,vol. 16, pp. 4551- 4568 ,(1977) , 10.1103/PHYSREVB.16.4551
C. Tiby, H.J. Lauter, A neutron scattering study of the structures and phase transitions of 36Ar submonolayers on grafoil Surface Science. ,vol. 117, pp. 277- 284 ,(1982) , 10.1016/0039-6028(82)90508-8
K. D. Gibson, S. J. Sibener, Determination of the surface phonon dispersion relations for monolayer, bilayer, trilayer, and thick Kr(111) films physisorbed on Ag(111) by inelastic He scattering. Physical Review Letters. ,vol. 55, pp. 1514- 1517 ,(1985) , 10.1103/PHYSREVLETT.55.1514
T.H. Ellis, G. Scoles, U. Valbusa, Surface vibrations of atoms physisorbed on a crystal surface: monolayer and bilayer xenon on (0001) graphite Chemical Physics Letters. ,vol. 94, pp. 247- 249 ,(1983) , 10.1016/0009-2614(83)87080-8
G. Brusdeylins, R. Bruce Doak, J. Peter Toennies, Observation of Surface Phonons in Inelastic Scattering of He Atoms from LiF(001) Crystal Surfaces Physical Review Letters. ,vol. 44, pp. 1417- 1420 ,(1980) , 10.1103/PHYSREVLETT.44.1417
G. Brusdeylins, R. Bruce Doak, J. Peter Toennies, High-resolution helium time-of-flight studies of Rayleigh surface-phonon dispersion curves of LiF, NaF, and KCl Physical Review B. ,vol. 27, pp. 3662- 3685 ,(1983) , 10.1103/PHYSREVB.27.3662