Flocculation Efficiency and Mechanism of Carbamazepine by Microbial Flocculant Extracted from Klebsiella pneumoniae J1.

作者: Jie Xing , Nanzhe Song , Xiangwei Chen , Ang Li , Hongwei Ni

DOI: 10.1155/2020/8811516

关键词: Klebsiella pneumoniaeNuclear chemistryKinetic equationsEffluentWastewaterSedimentation (water treatment)ChemistryCarbamazepineAdsorptionFlocculation

摘要: The microbial flocculant (MFX) extracted from Klebsiella pneumoniae J1 was used to remove carbamazepine in prepared wastewater and domestic sewage. influence factors flocculation mechanism were studied. optimal removal conditions for MFX pH of 7-8, 7 mL flocculant, 0.1 mL coagulant, 35°C, the rate reached 81.75%. efficient both sewage (75.03%) secondary sedimentation tank effluent (69.76%). pseudo-first-order kinetic equation fitted adsorption process better than pseudo-second-order equation, which suggested that not pure chemical adsorption. analysis floc size repulsive force between weakened under alkalescent conditions, can help growth coherence flocs increase efficiency. Enough dosage generate larger flocs, but excessive will decrease because electrostatic repulsion. 3D-EEM FTIR hydroxyl, amino, carboxyl played an important role carbamazepine. As eco-friendly highly has potential practical applications removal.

参考文章(32)
Jixian Yang, Wei Wei, Shanshan Pi, Fang Ma, Ang Li, Dan Wu, Jie Xing, Competitive adsorption of heavy metals by extracellular polymeric substances extracted from Klebsiella sp. J1. Bioresource Technology. ,vol. 196, pp. 533- 539 ,(2015) , 10.1016/J.BIORTECH.2015.08.011
Lilja Nielsen, Pengfei Zhang, Teresa J. Bandosz, Adsorption of carbamazepine on sludge/fish waste derived adsorbents: Effect of surface chemistry and texture Chemical Engineering Journal. ,vol. 267, pp. 170- 181 ,(2015) , 10.1016/J.CEJ.2014.12.113
Jie Xing, Ji-Xian Yang, Ang Li, Fang Ma, Ke-Xin Liu, Dan Wu, Wei Wei, Removal Efficiency and Mechanism of Sulfamethoxazole in Aqueous Solution by Bioflocculant MFX Journal of Automated Methods & Management in Chemistry. ,vol. 2013, pp. 568614- 568614 ,(2013) , 10.1155/2013/568614
Y.X. Zhao, B.Y. Gao, H.K. Shon, J.-H. Kim, Q.Y. Yue, Y. Wang, Floc characteristics of titanium tetrachloride (TiCl4) compared with aluminum and iron salts in humic acid–kaolin synthetic water treatment Separation and Purification Technology. ,vol. 81, pp. 332- 338 ,(2011) , 10.1016/J.SEPPUR.2011.07.041
Lilja Nielsen, Mark J. Biggs, William Skinner, Teresa J. Bandosz, The effects of activated carbon surface features on the reactive adsorption of carbamazepine and sulfamethoxazole Carbon. ,vol. 80, pp. 419- 432 ,(2014) , 10.1016/J.CARBON.2014.08.081
Jixian Yang, Dan Wu, Ang Li, Haijuan Guo, Han Chen, Shanshan Pi, Wei Wei, Fang Ma, The Addition of N-Hexanoyl-Homoserine Lactone to Improve the Microbial Flocculant Production of Agrobacterium tumefaciens Strain F2, an Exopolysaccharide Bioflocculant-Producing Bacterium. Applied Biochemistry and Biotechnology. ,vol. 179, pp. 728- 739 ,(2016) , 10.1007/S12010-016-2027-6
Zhaohui Yang, Min Li, Mingda Yu, Jing Huang, Haiyin Xu, Yan Zhou, Peipei Song, Rui Xu, A novel approach for methylene blue removal by calcium dodecyl sulfate enhanced precipitation and microbial flocculant GA1 flocculation Chemical Engineering Journal. ,vol. 303, pp. 1- 13 ,(2016) , 10.1016/J.CEJ.2016.05.101
Wei Wei, Qilin Wang, Ang Li, Jixian Yang, Fang Ma, Shanshan Pi, Dan Wu, Biosorption of Pb (II) from aqueous solution by extracellular polymeric substances extracted from Klebsiella sp. J1: adsorption behavior and mechanism assessment Scientific Reports. ,vol. 6, pp. 31575- 31575 ,(2016) , 10.1038/SREP31575
Jian Chen, Di Zhang, Huang Zhang, Saikat Ghosh, Bo Pan, Fast and slow adsorption of carbamazepine on biochar as affected by carbon structure and mineral composition. Science of The Total Environment. ,vol. 579, pp. 598- 605 ,(2017) , 10.1016/J.SCITOTENV.2016.11.052