Impulsive excitation of high vibrational states in I2–Xe complex on the electronic ground state
作者： Tiina Kiviniemi , Eero Hulkko , Mika Pettersson
DOI: 10.1016/J.CPLETT.2010.03.075
关键词: Excited state 、 Femtosecond 、 Ground state 、 Coherent anti-Stokes Raman spectroscopy 、 Atomic physics 、 Coherent control 、 Chemistry 、 Excitation 、 Raman spectroscopy
摘要: Abstract High vibrational states, up to ν = 22, are excited and investigated on the ground electronic state of a 1:1 I 2 –Xe complex isolated in solid Kr using femtosecond CARS technique spontaneous resonant Raman measurements. The results show that this system is promising candidate for investigations coherent control bimolecular reactions by wavepackets state.
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sci-hub.se 参考文章(11)
David J. Tannor, Ronnie Kosloff, Stuart A. Rice, Coherent pulse sequence induced control of selectivity of reactions: Exact quantum mechanical calculations Journal of Chemical Physics. ,vol. 85, pp. 5805- 5820 ,(1986) , 10.1063/1.451542
Tiina Kiviniemi, Toni Kiljunen, Mika Pettersson, Femtosecond coherent anti-Stokes Raman-scattering polarization beat spectroscopy of I2-Xe complex in solid krypton. Journal of Chemical Physics. ,vol. 125, pp. 164302- 164302 ,(2006) , 10.1063/1.2358987
D. Zeidler, S. Frey, W. Wohlleben, M. Motzkus, F. Busch, T. Chen, W. Kiefer, A. Materny, Optimal control of ground-state dynamics in polymers Journal of Chemical Physics. ,vol. 116, pp. 5231- 5235 ,(2002) , 10.1063/1.1450549
V. A. Apkarian, Comment on “Time-resolved laser induced harpoon reactions’’ Journal of Chemical Physics. ,vol. 106, pp. 5298- 5299 ,(1997) , 10.1063/1.473996
E. D. Potter, J. L. Herek, S. Pedersen, Q. Liu, A. H. Zewail, Femtosecond laser control of a chemical reaction Nature. ,vol. 355, pp. 66- 68 ,(1992) , 10.1038/355066A0
Tiina Kiviniemi, Eero Hulkko, Toni Kiljunen, Mika Pettersson, Iodine-benzene complex as a candidate for a real-time control of a bimolecular reaction. Spectroscopic studies of the properties of the 1:1 complex isolated in solid krypton. Journal of Physical Chemistry A. ,vol. 113, pp. 6326- 6333 ,(2009) , 10.1021/JP902012U
Tiina Kiviniemi, Jukka Aumanen, Pasi Myllyperkiö, V. A. Apkarian, Mika Pettersson, Time-resolved coherent anti-Stokes Raman-scattering measurements of I2 in solid Kr: Vibrational dephasing on the ground electronic state at 2.6–32 K The Journal of Chemical Physics. ,vol. 123, pp. 064509- 064509 ,(2005) , 10.1063/1.1990115
J. Almy, K. Kizer, R. Zadoyan, V. A. Apkarian, Resonant Raman, Hot, and Cold Luminescence of Iodine in Rare Gas Matrixes † Journal of Physical Chemistry A. ,vol. 104, pp. 3508- 3520 ,(2000) , 10.1021/JP993238M
R. Zadoyan, V.A. Apkarian, Femtochemistry of the liquid phase laser-induced harpoon reaction between Cl2 and Xe. Observation of bond formation in real time Chemical Physics Letters. ,vol. 206, pp. 475- 482 ,(1993) , 10.1016/0009-2614(93)80171-K
Marcos Dantus, Vadim V. Lozovoy, Experimental coherent laser control of physicochemical processes. Chemical Reviews. ,vol. 104, pp. 1813- 1859 ,(2004) , 10.1021/CR020668R