The long range transport of airborne material and its removal by deposition and washout - I. General considerations.

作者: R.A. Scriven , B.E.A. Fisher

DOI: 10.1016/0004-6981(75)90053-0

关键词: AerosolWind speedHydrologyRainoutAtmospheric sciencesDeposition (aerosol physics)Turbulent diffusionArea sourceOrder of magnitudeSea levelChemistry

摘要: Abstract The lifetime and decay distance of airborne pollution downwind from a large area source are examined assuming that the transport takes place between ground, or sea level, an inversion only removal mechanisms deposition washout by rain. Rainout chemical reactions not included in this preliminary account Part I concentrations taken to be uniform with height. detailed effects turbulent diffusion upon concentration profiles considered II. In absence rain decays exponentially, “decay” “travel” equal height multiplied ratio mean wind speed velocity. For sulphur dioxide passing over dry land is typically several hundred, so heights about 1 km give rise lifetimes day distances hundred kilometres. It shown as conditions vary there maximum rate at each which independent velocity decreases inversely source. When conversion sulphate aerosol place, again under assumption rainfall absent, corresponding life times increased order magnitude. extension analysis based on assumptions variable velocities indicated. moderate (1 mm h−1) present reduces On annual average basis remains comparable process, rates kilometres industrial areas being most small fraction g S m−2, per annum. effective process.

参考文章(20)
G. Nonhebel, Meteorology and atomic energy Atmospheric Environment (1967). ,vol. 3, pp. 497- 497 ,(1969) , 10.1016/0004-6981(69)90083-3
Volcanic dust in the atmosphere; with a chronology and assessment of its meteorological significance Philosophical transactions - Royal Society. Mathematical, physical and engineering sciences. ,vol. 266, pp. 425- 533 ,(1970) , 10.1098/RSTA.1970.0010
Philip Herries Gregory, The microbiology of the atmosphere ,(1961)
Variability and upper bounds for maximum ground level concentrations Philosophical Transactions of the Royal Society A. ,vol. 265, pp. 209- 220 ,(1969) , 10.1098/RSTA.1969.0050
H. Zeedijk, C.A. Velds, The transport of sulphur dioxide over a long distance Atmospheric Environment. ,vol. 7, pp. 849- 862 ,(1973) , 10.1016/0004-6981(73)90107-8
J. A. GARLAND, W. S. CLOUGH, D. FOWLER, Deposition of Sulphur Dioxide on Grass Nature. ,vol. 242, pp. 256- 257 ,(1973) , 10.1038/242256A0
Henning Rodhe, Christer Persson, Ove Åkesson, An investigation into regional transport of soot and sulfate aerosols Atmospheric Environment (1967). ,vol. 6, pp. 675- 693 ,(1972) , 10.1016/0004-6981(72)90025-X