Experimental Study of CO 2 Decomposition in a DC Micro-slit Sustained Glow Discharge Reactor

作者: Tao Ma , Hai-Xing Wang , Qi Shi , Shi-Ning Li , Su-Rong Sun

DOI: 10.1007/S11090-019-09996-3

关键词:

摘要: Carbon dioxide decomposition in a micro-slit sustained glow discharge reactor operated at low pressure of 8 Torr was studied experimentally. A specially designed with configuration, combined third electrode that allows the extraction electrons from discharge, used to extend volume discharge. It is found that, increase applied voltage electrode, both conversion fraction and energy efficiency CO2 increase. The three-electrode structure also extended parallel operation investigate effects voltage, flow rate, number units on decomposition. maximum 7.2% achieved rate 30 ml/min power 2.1 W for single unit, while three discharges connected parallel, 26.2% 2 ml/min 6.6 W. results demonstrate feasibility discharges, increasing increases high rates. better understanding physical chemical kinetic processes will lead optimization future reactors improve efficiency.

参考文章(76)
Alexander Fridman, Plasma Chemistry Cambridge University Press. ,(2008) , 10.1017/CBO9780511546075
Xiaofei Duan, Yanping Li, Wenjie Ge, Baowei Wang, Degradation of CO2 through dielectric barrier discharge microplasma Greenhouse Gases-Science and Technology. ,vol. 5, pp. 131- 140 ,(2015) , 10.1002/GHG.1425
Danhua Mei, Xinbo Zhu, Chunfei Wu, Bryony Ashford, Paul T. Williams, Xin Tu, Plasma-photocatalytic conversion of CO2 at low temperatures: Understanding the synergistic effect of plasma-catalysis Applied Catalysis B-environmental. ,vol. 182, pp. 525- 532 ,(2016) , 10.1016/J.APCATB.2015.09.052
R. Shrestha, R. B. Tyata, D. P. Subedi, Effect of Applied Voltage in Electron Density of Homogeneous Dielectric Barrier Discharge at Atmospherice Pressure The Himalayan Physics. ,vol. 4, pp. 10- 13 ,(2013) , 10.3126/HJ.V4I0.9418
Robert H. Stark, Karl H. Schoenbach, Direct current high-pressure glow discharges Journal of Applied Physics. ,vol. 85, pp. 2075- 2080 ,(2000) , 10.1063/1.369505
Kurt H. Becker, Brendan B. Godfrey, Erich E. Kunhardt, Mounir Laroussi, Lars D. Ludeking, Andreas A. Neuber, Edl Schamiloglu, Andrew J. Woods, Robert Barker Memorial Session: Leadership in Plasma Science and Applications IEEE Transactions on Plasma Science. ,vol. 43, pp. 914- 936 ,(2015) , 10.1109/TPS.2014.2378551
A.-A.H. Mohamed, R. Block, K.H. Schoenbach, Direct current glow discharges in atmospheric air IEEE Transactions on Plasma Science. ,vol. 30, pp. 182- 183 ,(2002) , 10.1109/TPS.2002.1003984
Tomáš Kozák, Annemie Bogaerts, Evaluation of the energy efficiency of CO 2 conversion in microwave discharges using a reaction kinetics model Plasma Sources Science and Technology. ,vol. 24, pp. 015024- ,(2014) , 10.1088/0963-0252/24/1/015024
Bing Qi, Jianjun Huang, Liang Gao, Yunming Qiu, None, Electron density measurements in an atmospheric pressure argon discharge by means of plasma radiation Physics of Plasmas. ,vol. 16, pp. 083301- ,(2009) , 10.1063/1.3200894
P Kurunczi, K.E Martus, K Becker, Neon excimer emission from pulsed high-pressure microhollow cathode discharge plasmas International Journal of Mass Spectrometry. ,vol. 223, pp. 37- 43 ,(2003) , 10.1016/S1387-3806(02)00778-9