X-ray scattering measurements of dissociation-induced metallization of dynamically compressed deuterium

作者: P. Davis , T. Döppner , J. R. Rygg , C. Fortmann , L. Divol

DOI: 10.1038/NCOMMS11189

关键词:

摘要: Hydrogen, the simplest element in universe, has a surprisingly complex phase diagram. Because of applications to planetary science, inertial confinement fusion and fundamental physics, its high-pressure properties have been subject intense study over past two decades. While sophisticated static experiments probed hydrogen's structure at ever higher pressures, studies examining higher-temperature regime using dynamic compression mostly limited optical measurement techniques. Here we present spectrally resolved x-ray scattering measurements from plasmons dynamically compressed deuterium. Combined with Compton scattering, velocity interferometry determine shock pressure mass density, this allows us extract ionization state as function compression. The onset occurs close where density functional theory-molecular dynamics (DFT-MD) simulations show molecular dissociation, suggesting hydrogen transitions insulating fluid conducting without passing through an intermediate atomic phase.

参考文章(55)
M. D. Knudson, M. P. Desjarlais, A. Becker, R. W. Lemke, K. R. Cochrane, M. E. Savage, D. E. Bliss, T. R. Mattsson, R. Redmer, Direct observation of an abrupt insulator-to-metal transition in dense liquid deuterium Science. ,vol. 348, pp. 1455- 1460 ,(2015) , 10.1126/SCIENCE.AAA7471
Nadine Nettelmann, Bastian Holst, André Kietzmann, Martin French, Ronald Redmer, David Blaschke, AB INITIO EQUATION OF STATE DATA FOR HYDROGEN, HELIUM, AND WATER AND THE INTERNAL STRUCTURE OF JUPITER The Astrophysical Journal. ,vol. 683, pp. 1217- 1228 ,(2008) , 10.1086/589806
S. H. Glenzer, G. Gregori, R. W. Lee, F. J. Rogers, S. W. Pollaine, O. L. Landen, Demonstration of spectrally resolved x-ray scattering in dense plasmas. Physical Review Letters. ,vol. 90, pp. 175002- ,(2003) , 10.1103/PHYSREVLETT.90.175002
Hugh F. Wilson, Burkhard Militzer, Rocky Core Solubility in Jupiter and Giant Exoplanets Physical Review Letters. ,vol. 108, pp. 111101- ,(2012) , 10.1103/PHYSREVLETT.108.111101
M. D. Knudson, D. L. Hanson, J. E. Bailey, C. A. Hall, J. R. Asay, C. Deeney, Principal Hugoniot, reverberating wave, and mechanical reshock measurements of liquid deuterium to 400 GPa using plate impact techniques Physical Review B. ,vol. 69, pp. 144209- ,(2004) , 10.1103/PHYSREVB.69.144209
M. D. Knudson, D. L. Hanson, J. E. Bailey, C. A. Hall, J. R. Asay, W. W. Anderson, Equation of state measurements in liquid deuterium to 70 GPa. Physical Review Letters. ,vol. 87, pp. 225501- ,(2001) , 10.1103/PHYSREVLETT.87.225501
W. J. Nellis, S. T. Weir, A. C. Mitchell, Minimum metallic conductivity of fluid hydrogen at 140 GPa (1.4 Mbar) Physical Review B. ,vol. 59, pp. 3434- 3449 ,(1999) , 10.1103/PHYSREVB.59.3434
S. H. Glenzer, O. L. Landen, P. Neumayer, R. W. Lee, K. Widmann, S. W. Pollaine, R. J. Wallace, G. Gregori, A. Höll, T. Bornath, R. Thiele, V. Schwarz, W.-D. Kraeft, R. Redmer, Observations of plasmons in warm dense matter. Physical Review Letters. ,vol. 98, pp. 065002- ,(2007) , 10.1103/PHYSREVLETT.98.065002
John P. Perdew, Kieron Burke, Matthias Ernzerhof, Generalized Gradient Approximation Made Simple Physical Review Letters. ,vol. 77, pp. 3865- 3868 ,(1996) , 10.1103/PHYSREVLETT.77.3865
A. L. Kritcher, P. Neumayer, J. Castor, T. Doppner, R. W. Falcone, O. L. Landen, H. J. Lee, R. W. Lee, E. C. Morse, A. Ng, S. Pollaine, D. Price, S. H. Glenzer, Ultrafast X-ray Thomson Scattering of Shock-Compressed Matter Science. ,vol. 322, pp. 69- 71 ,(2008) , 10.1126/SCIENCE.1161466