Optical second-order nonlinearity of the infrared transmitting 82GeS2∙18CdGa2S4 nanocrystallized chalcogenide glass

作者: Haizheng Tao , Changgui Lin , Shaoxuan Gu , Chengbin Jing , Xiujian Zhao

DOI: 10.1063/1.2754361

关键词:

摘要: The infrared (IR) transmitting nanocrystallized chalcogenide glass only containing α-CdGa2S4 IR nonlinear optical crystallites, which were confirmed by x-ray diffraction and Raman scattering measurements, was fabricated through the controllable nucleation crystallization of with composition 82GeS2∙18CdGa2S4 at a temperature 325°C far below transition (Tg:415°C) for long duration. A clear second harmonic generation (green light, 532nm) could be observed in transparent glass, demonstrating frequency-doubling function prepared composite material.

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