Epoxide pathways improve model predictions of isoprene markers and reveal key role of acidity in aerosol formation.

作者: Havala O. T. Pye , Robert W. Pinder , Ivan R. Piletic , Ying Xie , Shannon L. Capps

DOI: 10.1021/ES402106H

关键词:

摘要: Isoprene significantly contributes to organic aerosol in the southeastern United States where biogenic hydrocarbons mix with anthropogenic emissions. In this work, the Community …

参考文章(67)
T. S. Bates, B. K. Lamb, A. Guenther, J. Dignon, R. E. Stoiber, Sulfur Emissions to the Atmosphere from Natural Sources Journal of Atmospheric Chemistry. ,vol. 14, pp. 315- 337 ,(1992) , 10.1007/BF00115242
Xinrong Ren, William H Brune, Jingqiu Mao, Michael J Mitchell, Robert L Lesher, James B Simpas, Andrew R Metcalf, James J Schwab, Chenxia Cai, Yongquan Li, Kenneth L Demerjian, Henry D Felton, Garry Boynton, Allen Adams, Jacqueline Perry, Yi He, Xianliang Zhou, Jian Hou, Behavior of OH and HO2 in the winter atmosphere in New York City Atmospheric Environment. ,vol. 40, pp. 252- 263 ,(2006) , 10.1016/J.ATMOSENV.2005.11.073
Jason D. Surratt, Michael Lewandowski, John H. Offenberg, Mohammed Jaoui, Tadeusz E. Kleindienst, Edward O. Edney, John H. Seinfeld, Effect of acidity on secondary organic aerosol formation from isoprene. Environmental Science & Technology. ,vol. 41, pp. 5363- 5369 ,(2007) , 10.1021/ES0704176
A. H. Goldstein, C. D. Koven, C. L. Heald, I. Y. Fung, Biogenic carbon and anthropogenic pollutants combine to form a cooling haze over the southeastern United States Proceedings of the National Academy of Sciences of the United States of America. ,vol. 106, pp. 8835- 8840 ,(2009) , 10.1073/PNAS.0904128106
Ivan R. Piletic, Edward O. Edney, Libero J. Bartolotti, A computational study of acid catalyzed aerosol reactions of atmospherically relevant epoxides Physical Chemistry Chemical Physics. ,vol. 15, pp. 18065- 18076 ,(2013) , 10.1039/C3CP52851K
William M. Meylan, Philip H. Howard, Bond contribution method for estimating henry's law constants Environmental Toxicology and Chemistry. ,vol. 10, pp. 1283- 1293 ,(1991) , 10.1002/ETC.5620101007
T. L. Otte, J. E. Pleim, The Meteorology-Chemistry Interface Processor (MCIP) for the CMAQ modeling system: updates through MCIPv3.4.1 Geoscientific Model Development. ,vol. 3, pp. 243- 256 ,(2010) , 10.5194/GMD-3-243-2010
N. H. Robinson, J. F. Hamilton, J. D. Allan, B. Langford, D. E. Oram, Q. Chen, K. Docherty, D. K. Farmer, J. L. Jimenez, M. W. Ward, C. N. Hewitt, M. H. Barley, M. E. Jenkin, A. R. Rickard, S. T. Martin, G. McFiggans, H. Coe, Evidence for a significant proportion of Secondary Organic Aerosol from isoprene above a maritime tropical forest Atmospheric Chemistry and Physics. ,vol. 11, pp. 1039- 1050 ,(2011) , 10.5194/ACP-11-1039-2011
R. Locatelli, P. Bousquet, F. Chevallier, A. Fortems-Cheney, S. Szopa, M. Saunois, A. Agusti-Panareda, D. Bergmann, H. Bian, P. Cameron-Smith, M. P. Chipperfield, E. Gloor, S. Houweling, S. R. Kawa, M. Krol, P. K. Patra, R. G. Prinn, M. Rigby, R. Saito, C. Wilson, Impact of transport model errors on the global and regional methane emissions estimated by inverse modelling Atmospheric Chemistry and Physics. ,vol. 13, pp. 9917- 9937 ,(2013) , 10.5194/ACP-13-9917-2013
Y. Xie, F. Paulot, W. P. L. Carter, C. G. Nolte, D. J. Luecken, W. T. Hutzell, P. O. Wennberg, R. C. Cohen, R. W. Pinder, Understanding the impact of recent advances in isoprene photooxidation on simulations of regional air quality Atmospheric Chemistry and Physics. ,vol. 13, pp. 8439- 8455 ,(2013) , 10.5194/ACP-13-8439-2013