Wave Packet Dynamics in Ultrafast Spectroscopy of the Hydrated Electron
作者： A. Kummrow , M. F. Emde , A. Baltuška , M. S. Pshenichnikov , D. A. Wiersma
DOI: 10.1021/JP980254V
关键词:
摘要: Hydrated-electron dynamics is examined by frequency-resolved pump-probe experiments using pulses of 13 fs centered at 780 nm. A recurrence ~40 signifies a strong coupling the electronic transition to underdamped solvent motions. Wave packet launched pump pulse produces an ultrafast red-shift approximately 6500 cm-1. Gross features are analyzed two-level system.
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