Disentangling multipole resonances through a full x-ray polarization analysis

作者: C. Mazzoli , S. B. Wilkins , S. Di Matteo , B. Detlefs , C. Detlefs

DOI: 10.1103/PHYSREVB.76.195118

关键词:

摘要: Complete polarization analysis applied to resonant x-ray scattering at the Cr K edge in K2CrO4 shows that incident linearly polarized x rays can be converted into circularly by diffraction pre-edge (E=5994eV) . The physical mechanism behind this phenomenon is a subtle interference effect between purely dipole (E1-E1) and quadrupole (E2-E2) transitions, leading phase shift respective amplitudes. This may exploited disentangle two close-lying resonances appear as single peak conventional energy scan, way allowing one out identify different multipole order parameters involved.

参考文章(28)
Y. Murakami, H. Kawada, H. Kawata, M. Tanaka, T. Arima, Y. Moritomo, Y. Tokura, Direct Observation of Charge and Orbital Ordering in La 0.5 Sr 1.5 MnO 4 Physical Review Letters. ,vol. 80, pp. 1932- 1935 ,(1998) , 10.1103/PHYSREVLETT.80.1932
Y. Murakami, J. P. Hill, D. Gibbs, M. Blume, I. Koyama, M. Tanaka, H. Kawata, T. Arima, Y. Tokura, K. Hirota, Y. Endoh, Resonant X-Ray Scattering from Orbital Ordering in LaMnO 3 Physical Review Letters. ,vol. 81, pp. 582- 585 ,(1998) , 10.1103/PHYSREVLETT.81.582
Y. Joly, Grenier, J. E. Lorenzo, Resonant x-ray-diffraction study of the charge ordering in NaV 2 O 5 Physical Review B. ,vol. 68, pp. 104412- ,(2003) , 10.1103/PHYSREVB.68.104412
S. B. Wilkins, P. D. Hatton, M. D. Roper, D. Prabhakaran, A. T. Boothroyd, Soft X-ray resonant magnetic diffraction. Physical Review Letters. ,vol. 90, pp. 187201- ,(2003) , 10.1103/PHYSREVLETT.90.187201
S. B. Wilkins, P. D. Spencer, P. D. Hatton, S. P. Collins, M. D. Roper, D. Prabhakaran, A. T. Boothroyd, Direct observation of orbital ordering in La0.5Sr1.5MnO4 using soft x-ray diffraction. Physical Review Letters. ,vol. 91, pp. 167205- ,(2003) , 10.1103/PHYSREVLETT.91.167205
J. He, X. Yu, Y. Tokura, M. Kubota, T. Arima, Y. Kaneko, X-ray directional dichroism of a polar ferrimagnet. Physical Review Letters. ,vol. 92, pp. 137401- ,(2004) , 10.1103/PHYSREVLETT.92.137401
José Goulon, Chantal Goulon-Ginet, Andrei Rogalev, Vincent Gotte, Cécile Malgrange, Christian Brouder, Calogero R. Natoli, X-ray natural circular dichroism in a uniaxial gyrotropic single crystal of LiIO3 Journal of Chemical Physics. ,vol. 108, pp. 6394- 6403 ,(1998) , 10.1063/1.476046
S. Di Matteo, Y. Joly, C. R. Natoli, Detection of electromagnetic multipoles by x-ray spectroscopies Physical Review B. ,vol. 72, ,(2005) , 10.1103/PHYSREVB.72.144406
J. A. Paixão, C. Detlefs, M. J. Longfield, R. Caciuffo, P. Santini, N. Bernhoeft, J. Rebizant, G. H. Lander, Triple-q(-->) octupolar ordering in NpO2. Physical Review Letters. ,vol. 89, pp. 187202- ,(2002) , 10.1103/PHYSREVLETT.89.187202
S. Di Matteo, Y. Joly, A. Bombardi, L. Paolasini, F. de Bergevin, C. R. Natoli, Local chiral-symmetry breaking in globally centrosymmetric crystals. Physical Review Letters. ,vol. 91, pp. 257402- 257402 ,(2003) , 10.1103/PHYSREVLETT.91.257402