A test of optimal laser impulsion for controlling population within the Ns=1, Nr=5 polyad of 12C2H2

作者: Nathalie Vaeck , Michel Herman , Michèle Desouter-Lecomte , Ludovic Santos , David D.S. Perry

DOI: 10.1080/00268976.2015.1102980

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摘要: ABSTRACTOptimal control theory has been employed to populate separately two dark states of the acetylene polyad, Ns = 1 and Nr = 5, by indirect coupling via ground state. Relevant level energies transition dipole moments are extracted from experimental literature. The optimal pulses rather simple. evolution population is shown for duration process also field-free that follows control. One appears be a potential target realistic investigation because average Rabi oscillation remains high decoherence expected weak.

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