Monotonic convergent optimal control theory with strict limitations on the spectrum of optimized laser fields.

摘要: We present a modified optimal control scheme based on the Krotov method, which allows for strict limitations spectrum of optimized laser fields. A frequency constraint is introduced and derived mathematically correct, without losing monotonic convergence algorithm. The method guarantees close link to learning loop experiments demonstrated challenging nonresonant Raman transitions, are used implement set global quantum gates molecular vibrational qubits.