Movies of the Glass Transition

作者: M. D. Ediger

DOI: 10.1126/SCIENCE.287.5453.604

关键词:

摘要: The phenomenology of glass formation has been known for decades, but important questions regarding the heterogeneity and cooperativity molecular dynamics in glasses have remained inaccessible to experiments. Weeks et al . (page 627) Kegel van Blaaderen (14 January 2000, page 290) performed imaging studies a model glass-forming system consisting colloidal spheres suspended solvent. unprecedented detail these data may help resolve primary issue transition, namely cause slow dynamics.

参考文章(10)
Maria Luisa Ferrer, Christopher Lawrence, Berj G. Demirjian, Daniel Kivelson, Christiane Alba-Simionesco, Gilles Tarjus, Supercooled liquids and the glass transition: Temperature as the control variable The Journal of Chemical Physics. ,vol. 109, pp. 8010- 8015 ,(1998) , 10.1063/1.477448
Eric R Weeks, John C Crocker, Andrew C Levitt, Andrew Schofield, David A Weitz, Three-Dimensional Direct Imaging of Structural Relaxation Near the Colloidal Glass Transition Science. ,vol. 287, pp. 627- 631 ,(2000) , 10.1126/SCIENCE.287.5453.627
Chia-Ying Wang, M. D. Ediger, How long do regions of different dynamics persist in supercooled o-terphenyl? Journal of Physical Chemistry B. ,vol. 103, pp. 4177- 4184 ,(1999) , 10.1021/JP984149X
W. van Megen, S. M. Underwood, Glass transition in colloidal hard spheres: Mode-coupling theory analysis. Physical Review Letters. ,vol. 70, pp. 2766- 2769 ,(1993) , 10.1103/PHYSREVLETT.70.2766
Walter. Kauzmann, The Nature of the Glassy State and the Behavior of Liquids at Low Temperatures. Chemical Reviews. ,vol. 43, pp. 219- 256 ,(1948) , 10.1021/CR60135A002
Hans Sillescu, Heterogeneity at the glass transition: a review Journal of Non-crystalline Solids. ,vol. 243, pp. 81- 108 ,(1999) , 10.1016/S0022-3093(98)00831-X
Claudio Donati, Sharon C. Glotzer, Peter H. Poole, Walter Kob, Steven J. Plimpton, Spatial correlations of mobility and immobility in a glass-forming Lennard-Jones liquid Physical Review E. ,vol. 60, pp. 3107- 3119 ,(1999) , 10.1103/PHYSREVE.60.3107
Willem K Kegel, and Alfons van Blaaderen, Direct Observation of Dynamical Heterogeneities in Colloidal Hard-Sphere Suspensions Science. ,vol. 287, pp. 290- 293 ,(2000) , 10.1126/SCIENCE.287.5451.290
William E Moerner, Michel Orrit, Illuminating Single Molecules in Condensed Matter Science. ,vol. 283, pp. 1670- 1676 ,(1999) , 10.1126/SCIENCE.283.5408.1670