Magnetic circular dichroism in resonant x-ray emission from impurities: Results at the L-2,(3) edges of Mn in Ni

作者: F. Borgatti , P. Ferriani , G. Ghringhelli , A. Tagliaferri , B. De Michelis

DOI: 10.1103/PHYSREVB.65.094406

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摘要: We present a study of Mn magnetic impurities (about 2%) in Ni with resonant x-ray emission spectroscopy excited at the L 2 . 3 edges using circularly polarized x rays incident almost parallel/antiparallel to magnetization. The results are discussed jointly absorption circular dichroism and complemented elastic reflectivity measurements. Moreover, we show that is particularly suitable impurity problem, since self-absorption/saturation corrections measurements rather limited. problem treated also theoretically full multiplet splitting calculation single + (3d 5 ) ion cubic crystal field. theory reproduces satisfactorily all experimental trends features dispersing photon energy whole region, whereas it not adequate just below excitation. joint use allows us extract nondispersive component from measured spectra. It shown this does correlate directly 3d-Mn local density states. general implications discussed.

参考文章(35)
P. Strange, P. J. Durham, B. L. Gyorffy, Dichroic x-ray fluorescence Physical Review Letters. ,vol. 67, pp. 3590- 3593 ,(1991) , 10.1103/PHYSREVLETT.67.3590
C. F. Hague, J-M. Mariot, P. Strange, P. J. Durham, B. L. Gyorffy, Observation of magnetic circular dichroism in Fe L2,3 x-ray-fluorescence spectra. Physical Review B. ,vol. 48, pp. 3560- 3562 ,(1993) , 10.1103/PHYSREVB.48.3560
Michio Tokuyama, Irwin Oppenheim, Dynamics of hard-sphere suspensions Physical Review E. ,vol. 50, pp. R16- R19 ,(1994) , 10.1103/PHYSREVE.50.R16
C. F. Hague, J.-M. Mariot, G. Y. Guo, K. Hricovini, G. Krill, Coster-Kronig contributions to magnetic circular dichroism in the L2,3 x-ray fluorescence of iron. Physical Review B. ,vol. 51, pp. 1370- 1373 ,(1995) , 10.1103/PHYSREVB.51.1370
A. Báder, L. Sarkadi, L. Víkor, M. Kuzel, P. A. Závodszky, T. Jalowy, K. O. Groeneveld, P. A. Macri, R. O. Barrachina, Observation of low-lying resonance states of He{sup {minus}} at the 2 {sup 1}S and 2 {sup 3}S He thresholds Physical Review A. ,vol. 55, ,(1997) , 10.1103/PHYSREVA.55.R14
S Eisebitt, J Lüning, J.-E Rubensson, D Schmitz, S Blügel, W Eberhardt, Dichroism and spin information in soft X-ray emission Solid State Communications. ,vol. 104, pp. 173- 177 ,(1997) , 10.1016/S0038-1098(97)00108-7
L. Braicovich, C. Dallera, G. Ghiringhelli, N.B. Brookes, J.B. Goedkoop, Magnetic circular dichroism in resonant soft X-ray inelastic scattering: The recovery of the useful information from the raw data Solid State Communications. ,vol. 105, pp. 263- 267 ,(1998) , 10.1016/S0038-1098(97)10108-9
L.-C Duda, Magnetic circular dichroism in soft X-ray emission of itinerant and localized magnets Journal of Electron Spectroscopy and Related Phenomena. ,vol. 110, pp. 287- 304 ,(2000) , 10.1016/S0368-2048(00)00169-9
M.V Yablonskikh, V.I Grebennikov, Yu.M Yarmoshenko, E.Z Kurmaev, S.M Butorin, L.-C Duda, C Sȧthe, T Käämbre, M Magnuson, J Nordgren, S Plogmann, M Neumann, Magnetic circular dichroism in X-ray fluorescence of Heusler alloys at threshold excitation Solid State Communications. ,vol. 117, pp. 79- 82 ,(2000) , 10.1016/S0038-1098(00)00415-4
M. V. Yablonskikh, Yu. M. Yarmoshenko, V. I. Grebennikov, E. Z. Kurmaev, S. M. Butorin, L.-C. Duda, J. Nordgren, S. Plogmann, M. Neumann, Origin of magnetic circular dichroism in soft x-ray fluorescence of Heusler alloys at threshold excitation Physical Review B. ,vol. 63, pp. 235117- ,(2001) , 10.1103/PHYSREVB.63.235117