Enhanced hole injection in organic light-emitting diodes utilizing a copper iodide-doped hole injection layer

作者: Meiling Shan , Haipeng Jiang , Yu Guan , Dongsu Sun , Yu Wang

DOI: 10.1039/C6RA28644E

关键词:

摘要: We have demonstrated organic light-emitting diodes (OLEDs) by incorporating copper iodide (CuI) in 4,4′,4′′-tris(N-3-methylphenyl-N-phenyl-amino)triphenylamine (m-MTDATA) as a hole injection layer (HIL) based on the emitting system of C545T–Alq3. The device with CuI-doped m-MTDATA HIL shows very low operating voltage about 4.26 and 5.70 V for 1000 10 000 cd m−2, respectively, which reveals great improvement over undoped (4.85 m−2 7.72 m−2). Furthermore, exhibits maximum power efficiency 5.88 lm W−1, 58% higher than that corresponding (3.71 W−1). improved performance could be attributed to enhanced transport due generation free charge carriers transfer from CuI molecules, leading an increase electrical conductivity formation ohmic contact at ITO/HIL interface.

参考文章(34)
Ya-Hui Duan, Yu Duan, Xiao Wang, Dan Yang, Yong-Qiang Yang, Ping Chen, Feng-Bo Sun, Kai-Wen Xue, Yi Zhao, Highly flexible peeled-off silver nanowire transparent anode using in organic light-emitting devices Applied Surface Science. ,vol. 351, pp. 445- 450 ,(2015) , 10.1016/J.APSUSC.2015.05.161
Qisheng Zhang, Bo Li, Shuping Huang, Hiroko Nomura, Hiroyuki Tanaka, Chihaya Adachi, Efficient blue organic light-emitting diodes employing thermally activated delayed fluorescence Nature Photonics. ,vol. 8, pp. 326- 332 ,(2014) , 10.1038/NPHOTON.2014.12
Chimed Ganzorig, Masamichi Fujihira, Improved drive voltages of organic electroluminescent devices with an efficient p-type aromatic diamine hole-injection layer Applied Physics Letters. ,vol. 77, pp. 4211- 4213 ,(2000) , 10.1063/1.1331640
Sebastian Reineke, Frank Lindner, Gregor Schwartz, Nico Seidler, Karsten Walzer, Björn Lüssem, Karl Leo, White organic light-emitting diodes with fluorescent tube efficiency Nature. ,vol. 459, pp. 234- 238 ,(2009) , 10.1038/NATURE08003
S. A. Choulis, V.-E. Choong, A. Patwardhan, M. K. Mathai, F. So, Interface Modification to Improve Hole-Injection Properties in Organic Electronic Devices** Advanced Functional Materials. ,vol. 16, pp. 1075- 1080 ,(2006) , 10.1002/ADFM.200500443
X. Zhou, J. Blochwitz, M. Pfeiffer, A. Nollau, T. Fritz, K. Leo, Enhanced Hole Injection into Amorphous Hole-Transport Layers of Organic Light-Emitting Diodes Using Controlled p-Type Doping Advanced Functional Materials. ,vol. 11, pp. 310- 314 ,(2001) , 10.1002/1616-3028(200108)11:4<310::AID-ADFM310>3.0.CO;2-D
Hany Aziz, Zoran D Popovic, Nan-Xing Hu, Ah-Mee Hor, Gu Xu, Degradation Mechanism of Small Molecule-Based Organic Light-Emitting Devices Science. ,vol. 283, pp. 1900- 1902 ,(1999) , 10.1126/SCIENCE.283.5409.1900
Won-Ju Shin, Je-Yun Lee, Jae Chang Kim, Tae-Hoon Yoon, Tae-Shick Kim, Ok-Keun Song, Bulk and interface properties of molybdenum trioxide-doped hole transporting layer in organic light-emitting diodes Organic Electronics. ,vol. 9, pp. 333- 338 ,(2008) , 10.1016/J.ORGEL.2007.12.001
Hongmei Zhang, Qiang Fu, Wenjin Zeng, Dongge Ma, High-efficiency fluorescent organic light-emitting diodes with MoO3 and PEDOT : PSS composition film as a hole injection layer Journal of Materials Chemistry C. ,vol. 2, pp. 9620- 9624 ,(2014) , 10.1039/C4TC01310G