Influence of CeO2 nanoparticles on viscoelastic properties of sludge: Role of extracellular polymeric substances

作者: Guoxiang You , Peifang Wang , Jun Hou , Chao Wang , Lingzhan Miao

DOI: 10.1016/J.ENVRES.2018.07.005

关键词:

摘要: Abstract Cerium oxide nanoparticles (CeO2 NPs) affected the production of extracellular polymeric substances (EPSs), and thus might bring challenges for sludge pumping mixing. In present study, we investigated rheological behavior before after extraction different EPSs fractions under various CeO2 NPs concentrations. It was found that removal loosely bound (LB-EPSs) could affect shear stress (τ) apparent viscosity (η), changes were dependent on The tightly (TB-EPSs) either with or without addition significantly decreased yield (τy) limiting (η∞). Furthermore, dynamic (strain, frequency time) sweep measurements proved storage modulus (G') TB-EPSs, indicating weakened elastic solid-like properties. fluctuated content polysaccharide in LB-EPSs increased amount protein TB-EPSs likely to contribute variation viscoelastic behaviors respectively. addition, properties also related zeta potential, particle size key organic matters (104–106 Da) stratified EPSs. These results significant take advantages treatment presence NPs.

参考文章(36)
Guoxiang You, Jun Hou, Yi Xu, Chao Wang, Peifang Wang, Lingzhan Miao, Yanhui Ao, Yi Li, Bowen Lv, Effects of CeO2 nanoparticles on production and physicochemical characteristics of extracellular polymeric substances in biofilms in sequencing batch biofilm reactor Bioresource Technology. ,vol. 194, pp. 91- 98 ,(2015) , 10.1016/J.BIORTECH.2015.07.006
Jun Hou, Guoxiang You, Yi Xu, Chao Wang, Peifang Wang, Lingzhan Miao, Yanhui Ao, Yi Li, Bowen Lv, Effects of CeO2 nanoparticles on biological nitrogen removal in a sequencing batch biofilm reactor and mechanism of toxicity. Bioresource Technology. ,vol. 191, pp. 73- 78 ,(2015) , 10.1016/J.BIORTECH.2015.04.123
Maria Ruiz-Hernando, Jordi Labanda, Joan Llorens, Structural model to study the influence of thermal treatment on the thixotropic behaviour of waste activated sludge Chemical Engineering Journal. ,vol. 262, pp. 242- 249 ,(2015) , 10.1016/J.CEJ.2014.09.097
Ling-Li Li, Zhong-Hua Tong, Cai-Yun Fang, Jian Chu, Han-Qing Yu, Response of anaerobic granular sludge to single-wall carbon nanotube exposure. Water Research. ,vol. 70, pp. 1- 8 ,(2015) , 10.1016/J.WATRES.2014.11.042
Dongqin Yuan, Yili Wang, Influence of extracellular polymeric substances on rheological properties of activated sludge Biochemical Engineering Journal. ,vol. 77, pp. 208- 213 ,(2013) , 10.1016/J.BEJ.2013.06.011
Stephan Wagner, Andreas Gondikas, Elisabeth Neubauer, Thilo Hofmann, Frank von der Kammer, Spot the Difference: Engineered and Natural Nanoparticles in the Environment—Release, Behavior, and Fate Angewandte Chemie. ,vol. 53, pp. 12398- 12419 ,(2014) , 10.1002/ANIE.201405050
S LYKO, T WINTGENS, D ALHALBOUNI, S BAUMGARTEN, D TACKE, K DRENSLA, A JANOT, W DOTT, J PINNEKAMP, T MELIN, Long-term monitoring of a full-scale municipal membrane bioreactor—Characterisation of foulants and operational performance Journal of Membrane Science. ,vol. 317, pp. 78- 87 ,(2008) , 10.1016/J.MEMSCI.2007.07.008
E. Dieudé-Fauvel, P. Héritier, M. Chanet, R. Girault, D. Pastorelli, E. Guibelin, J.C. Baudez, Modelling the rheological properties of sludge during anaerobic digestion in a batch reactor by using electrical measurements. Water Research. ,vol. 51, pp. 104- 112 ,(2014) , 10.1016/J.WATRES.2013.12.018