Growth mechanisms of epitaxial metallic oxide SrRuO3 thin films studied by scanning tunneling microscopy

作者: R. A. Rao , Q. Gan , C. B. Eom

DOI: 10.1063/1.119616

关键词:

摘要: We report the deliberately controlled growth of epitaxial metallic oxide SrRuO3 thin films in three distinctly different modes. Scanning tunneling microscopy and x-ray diffraction indicate that mechanism for on exact (001) SrTiO3 substrates is two-dimensional nucleation, which results a two domain in-plane structure. As miscut angle vicinal increased, changes to step flow leads single films. Films LaAlO3 have an incoherent three-dimensional island due large lattice mismatch, resulting bulk-like lattice. The vast difference mechanisms these corresponding their electrical transport magnetic behavior. Such nanoscale control mechanism, surface morphology, structure can be very important fabrication novel perovskite devices.

参考文章(10)
The Growth of Crystals and the Equilibrium Structure of their Surfaces Philosophical transactions - Royal Society. Mathematical, physical and engineering sciences. ,vol. 243, pp. 299- 358 ,(1951) , 10.1098/RSTA.1951.0006
C. GERBER, D. ANSELMETTI, J. G. BEDNORZ, J. MANNHART, D. G. SCHLOM, Screw dislocations in high- T c films Nature. ,vol. 350, pp. 279- 280 ,(1991) , 10.1038/350279A0
C. B. Eom, R. J. Cava, R. M. Fleming, J. M. Phillips, R. B. vanDover, J. H. Marshall, J. W. P. Hsu, J. J. Krajewski, W. F. Peck, Single-Crystal Epitaxial Thin Films of the Isotropic Metallic Oxides Sr1–xCaxRuO3 (0 ≤ x ≤ 1) Science. ,vol. 258, pp. 1766- 1769 ,(1992) , 10.1126/SCIENCE.258.5089.1766
T. L. Hylton, M. R. Beasley, Flux-pinning mechanisms in thin films of YBa2Cu3Ox. Physical Review B. ,vol. 41, pp. 11669- 11672 ,(1990) , 10.1103/PHYSREVB.41.11669
M. Kawasaki, K. Takahashi, T. Maeda, R. Tsuchiya, M. Shinohara, O. Ishiyama, T. Yonezawa, M. Yoshimoto, H. Koinuma, Atomic Control of the SrTiO3 Crystal Surface Science. ,vol. 266, pp. 1540- 1542 ,(1994) , 10.1126/SCIENCE.266.5190.1540
M. HAWLEY, I. D. RAISTRICK, J. G. BEERY, R. J. HOULTON, Growth Mechanism of Sputtered Films of YBa2Cu3O7 Studied by Scanning Tunneling Microscopy Science. ,vol. 251, pp. 1587- 1589 ,(1991) , 10.1126/SCIENCE.251.5001.1587
J. Z. Sun, W. J. Gallagher, P. R. Duncombe, L. Krusin‐Elbaum, R. A. Altman, A. Gupta, Yu Lu, G. Q. Gong, Gang Xiao, Observation of large low‐field magnetoresistance in trilayer perpendicular transport devices made using doped manganate perovskites Applied Physics Letters. ,vol. 69, pp. 3266- 3268 ,(1996) , 10.1063/1.118031
T. Haage, Q. D. Jiang, M. Cardona, H.‐U. Habermeier, J. Zegenhagen, Direct scanning tunneling microscopy observation of non‐unit‐cell growth of YBa2Cu3O7−δ thin films Applied Physics Letters. ,vol. 68, pp. 2427- 2429 ,(1996) , 10.1063/1.116156
Q. Gan, R. A. Rao, C. B. Eom, Control of the growth and domain structure of epitaxial SrRuO3 thin films by vicinal (001) SrTiO3 substrates Applied Physics Letters. ,vol. 70, pp. 1962- 1964 ,(1997) , 10.1063/1.118792
VC Matijasevic, B Ilge, B Stäuble-Pümpin, G Rietveld, F Tuinstra, JE Mooij, None, Nucleation of a complex oxide during epitaxial film growth: SmBa2Cu3Oy on SrTiO3 Physical Review Letters. ,vol. 76, pp. 4765- 4768 ,(1996) , 10.1103/PHYSREVLETT.76.4765