Photoionization of small sodium-doped acetic acid clusters.
作者： Piotr W. Forysinski , Philipp Zielke , David Luckhaus , Jennifer Corbett , Ruth Signorell
DOI: 10.1063/1.3559464
关键词:
摘要: The uptake of sodium and the fragmentation before after “soft” photoionization with ultraviolet light are investigated for small acetic acid clusters. clusters generated in a supersonic expansion ionized doping pick-up chamber. composition bare molecular beam is determined independently from complementary experiments using extreme light. experimental results analyzed help density functional calculations energetics statistical adiabatic channel kinetics. study demonstrates that detected ions originate neutral as well ionic state, particular pathway strongly depends on cluster size.
scitation.org
harvard.edu
aip.org 
sci-hub.se 参考文章(32)
Peter A. Kollman, Norman L. Allinger, Henry F. Iii Schaefer, Peter R. Schreiner, Johann Gasteiger, Terry W. Clark, Encyclopedia of computational chemistry ,(1998)
Martin Quack, J��rgen Troe, Statistical Adiabatic Channel Models Encyclopedia of Computational Chemistry. ,(2002) , 10.1002/0470845015.CSA025
Orest Dorosh, Ewa Białkowska-Jaworska, Zbigniew Kisiel, Lech Pszczółkowski, New measurements and global analysis of rotational spectra of Cl-, Br-, and I-benzene: Spectroscopic constants and electric dipole moments Journal of Molecular Spectroscopy. ,vol. 246, pp. 228- 232 ,(2007) , 10.1016/J.JMS.2007.09.010
Xianzhao Peng, Wei Kong, Zero energy kinetic electron and mass analyzed threshold ionization spectroscopy of Na⋅(NH3)n (n=1, 2, and 4) complexes Journal of Chemical Physics. ,vol. 117, pp. 9306- 9315 ,(2002) , 10.1063/1.1516796
Bing Gao, Zhi-Feng Liu, Ionization induced relaxation in solvation structure: a comparison between Na(H2O)n and Na(NH3)n. Journal of Chemical Physics. ,vol. 126, pp. 084501- ,(2007) , 10.1063/1.2464109
C. P. Schulz, R. Haugst�tter, H. -U. Tittes, I. V. Hertel, Free sodium-water clusters: photoionisation studies in a pulsed molecular beam source European Physical Journal D. ,vol. 10, pp. 279- 290 ,(1988) , 10.1007/BF01384862
Ingo Dauster, Martin A. Suhm, Udo Buck, Thomas Zeuch, Experimental and theoretical study of the microsolvation of sodium atoms in methanol clusters: differences and similarities to sodium-water and sodium-ammonia. Physical Chemistry Chemical Physics. ,vol. 10, pp. 83- 95 ,(2008) , 10.1039/B711568G
C. Nitsch, C. P. Schulz, A. Gerber, W. Zimmermann-Edling, I. V. Hertel, Photoionization studies of free sodium ammonia clusters European Physical Journal D. ,vol. 22, pp. 651- 658 ,(1992) , 10.1007/BF01426368
Piotr W. Forysinski, Philipp Zielke, David Luckhaus, Ruth Signorell, PFI-ZEKE photoelectron spectrum of CH2F2, ionisation potential and ionic fragmentation appearance potentials Physical Chemistry Chemical Physics. ,vol. 12, pp. 3121- 3130 ,(2010) , 10.1039/B922298G
Philipp Zielke, Piotr W. Forysinski, David Luckhaus, Ruth Signorell, Adiabatic ionization potential of acetic acid and torsional dynamics of its cation Journal of Chemical Physics. ,vol. 130, pp. 211101- 211101 ,(2009) , 10.1063/1.3149802