Effect of mechanical constraint on the dielectric and piezoelectric behavior of epitaxial Pb(Mg1/3Nb2/3)O3(90%)–PbTiO3(10%) relaxor thin films

作者: V. Nagarajan , C. S. Ganpule , B. Nagaraj , S. Aggarwal , S. P. Alpay

DOI: 10.1063/1.125576

关键词:

摘要: The effect of heteroepitaxy-induced constraint on the structure and piezoelectric properties relaxor ferroelectric lead magnesium niobate–lead titanate (PMN–PT) were investigated. Relaxor PMN–PT epitaxial thin films with oxide electrodes grown by pulsed-laser deposition (100) LaAlO3 substrates. We observe a systematic decrease in phase transition temperature (temperature at which maximum dielectric response occurs), from around 250 to 60 °C as thickness is increased 100 400 nm. This accompanied an increase relative constant (er), measured room 10 kHz, 300 2000. coefficient d33 using scanned probe microscope, almost order magnitude increasing film thickness.

参考文章(13)
Z. Kighelman, D. Damjanovic, A. Seifert, L. Sagalowicz, N. Setter, Relaxor behavior and electromechanical properties of Pb(Mg1/3Nb2/3)O3 thin films Applied Physics Letters. ,vol. 73, pp. 2281- 2283 ,(1998) , 10.1063/1.121702
Shoichiro Nomura, Kenji Uchino, Electrostrictive effect in Pb(Mg1/3Nb2/3)O3-type materials Ferroelectrics. ,vol. 41, pp. 117- 132 ,(1982) , 10.1080/00150198208210614
Dan Lavric, Rajesh A. Rao, Qing Gan, J. J. Krajewski, Chang-Beom Eom, Epitaxial thin film heterostructures of relaxor ferroelectric Pb(Mg1/3Nb2/3)O3-PbTiO3 Integrated Ferroelectrics. ,vol. 21, pp. 499- 509 ,(1998) , 10.1080/10584589808202090
G. Catalan, M. H. Corbett, R. M. Bowman, J. M. Gregg, Influence of oxygen content on dielectric and electromechanical properties of Pb(Mg1/3Nb2/3)O3 thin films Applied Physics Letters. ,vol. 74, pp. 3035- 3037 ,(1999) , 10.1063/1.124056
J.-P. Maria, W. Hackenberger, S. Trolier-McKinstry, PHASE DEVELOPMENT AND ELECTRICAL PROPERTY ANALYSIS OF PULSED LASER DEPOSITED PB(MG1/3NB2/3)O3-PBTIO3 (70/30) EPITAXIAL THIN FILMS Journal of Applied Physics. ,vol. 84, pp. 5147- 5154 ,(1998) , 10.1063/1.368809
Jun Kuwata, Kenji Uchino, Shoichiro Nomura, Electrostrictive Coefficients of Pb(Mg1/3Nb2/3)O3Ceramics Japanese Journal of Applied Physics. ,vol. 19, pp. 2099- 2103 ,(1980) , 10.1143/JJAP.19.2099
Yutaka Takeshima, Kosuke Shiratsuyu, Hiroshi Takagi, Kunisaburo Tomono, Preparation of Lead Magnesium Niobate Titanate Thin Films by Chemical Vapor Deposition Japanese Journal of Applied Physics. ,vol. 34, pp. 5083- 5085 ,(1995) , 10.1143/JJAP.34.5083
R. Ramesh, C. S. Ganpule, A. Stanishevsky, Q. Su, S. Aggarwal, J. Melngailis, E. Williams, Scaling of ferroelectric properties in thin films Applied Physics Letters. ,vol. 75, pp. 409- 411 ,(1999) , 10.1063/1.124391
Q. M. Zhang, J. Zhao, Polarization responses in lead magnesium niobate based relaxor ferroelectrics Applied Physics Letters. ,vol. 71, pp. 1649- 1651 ,(1997) , 10.1063/1.119784
JA Christman, H Maiwa, S-H Kim, AI Kingon, RJ Nemanich, Piezoelectric measurements with atomic force microscopy Applied Physics Letters. ,vol. 73, pp. 3851- 3853 ,(1998) , 10.1063/1.122914