The research of photocatalytic activity on Si doped TiO 2 nanotubes

作者: Jun Xiao , Zhanchang Pan , Bo Zhang , Gen Liu , Huangchu Zhang

DOI: 10.1016/J.MATLET.2016.10.097

关键词:

摘要: Abstract Pure TiO 2 nanotubes (TiO NTs) and Si-doped NTs (Si–TiO were prepared by one-step solvothermal procedure using titanium oxysulfate tetraethoxysilane as silicon sources, respectively. The structure morphology of the samples characterized X-ray diffraction (XRD) Scanning electron microscopy (SEM). Energy Dispersive Spectrometer (EDS) photoelectron spectroscopy (XPS) showed that introduction Si into could be controlled successfully. result N absorption-desorption (BET) displayed 5% Si–TiO had highest specific surface areas among all samples. Notably, UV–Vis absorption spectra test a much higher photocatalytic activity compared with other samples, exhibited remarkable red-shift intensity appeared under UV irradiation. Therefore, can greatly improved suitable amount doping.

参考文章(14)
Mechthild Lübke, Ian Johnson, Neel M. Makwana, Dan Brett, Paul Shearing, Zhaolin Liu, Jawwad A. Darr, High power TiO2 and high capacity Sn-doped TiO2 nanomaterial anodes for lithium-ion batteries Journal of Power Sources. ,vol. 294, pp. 94- 102 ,(2015) , 10.1016/J.JPOWSOUR.2015.06.039
Lihong Wu, Yifeng Zhou, Wangyan Nie, Linyong Song, Pengpeng Chen, Synthesis of highly monodispersed teardrop-shaped core–shell SiO2/TiO2 nanoparticles and their photocatalytic activities Applied Surface Science. ,vol. 351, pp. 320- 326 ,(2015) , 10.1016/J.APSUSC.2015.05.152
Youjun Yan, Xiaoqing Qiu, Hui Wang, Liping Li, Xianzhi Fu, Ling Wu, Guangshe Li, Synthesis of titanate/anatase composites with highly photocatalytic decolorization of dye under visible light irradiation Journal of Alloys and Compounds. ,vol. 460, pp. 491- 495 ,(2008) , 10.1016/J.JALLCOM.2007.05.086
Ali Beitollahi, Amir Hossein Haj Daie, Leyla Samie, Mohammad Mehdi Akbarnejad, Synthesis and characterization of mesoporous TiO2 assembled as microspheres Journal of Alloys and Compounds. ,vol. 490, pp. 311- 317 ,(2010) , 10.1016/J.JALLCOM.2009.10.002
Y ZHANG, X LI, D CHEN, N MA, X HUA, H WANG, Si doping effects on the photocatalytic activity of TiO2 nanotubes film prepared by an anodization process Scripta Materialia. ,vol. 60, pp. 543- 546 ,(2009) , 10.1016/J.SCRIPTAMAT.2008.12.004
Chuen-Shii Chou, Ming-Geng Guo, Kuan-Hung Liu, Yi-Siang Chen, Preparation of TiO2 particles and their applications in the light scattering layer of a dye-sensitized solar cell Applied Energy. ,vol. 92, pp. 224- 233 ,(2012) , 10.1016/J.APENERGY.2011.10.038
R. Vasilić, S. Stojadinović, N. Radić, P. Stefanov, Z. Dohčević-Mitrović, B. Grbić, One-step preparation and photocatalytic performance of vanadium doped TiO2 coatings Materials Chemistry and Physics. ,vol. 151, pp. 337- 344 ,(2015) , 10.1016/J.MATCHEMPHYS.2014.11.077
Babak Mazinani, Abdul Kadir Masrom, Ali Beitollahi, Rafael Luque, Photocatalytic activity, surface area and phase modification of mesoporous SiO2–TiO2 prepared by a one-step hydrothermal procedure Ceramics International. ,vol. 40, pp. 11525- 11532 ,(2014) , 10.1016/J.CERAMINT.2014.03.071
Zhenfeng Bian, Jian Zhu, Fenglei Cao, Yuning Huo, Yunfeng Lu, Hexing Li, Solvothermal synthesis of well-defined TiO2 mesoporous nanotubes with enhanced photocatalytic activity Chemical Communications. ,vol. 46, pp. 8451- 8453 ,(2010) , 10.1039/C0CC02998J